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Absorbent used for removing dioxin in garbage incineration exhaust gas, and preparation method and application thereof

A waste incineration and dioxin technology, applied in separation methods, chemical instruments and methods, and other chemical processes, can solve problems such as complexity, high price of activated carbon, secondary pollution follow-up treatment, etc., and achieve simple preparation and good industrialization The effect of applying the foreground

Active Publication Date: 2012-12-19
安徽力奥环境新材料有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] The purpose of the present invention is to provide a kind of attapulgite clay composite adsorbent for efficiently removing dioxins in waste incineration waste gas, and to prepare for the high price of activated carbon in the existing activated carbon adsorption process, secondary pollution and complicated subsequent treatment. Method and its application

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0019] Weigh 4000.0g of attapulgite clay with a particle size of 3mm to 5mm, add 400.0g of 90% sulfuric acid aqueous solution, and activate it at a reaction temperature of 60°C for 20 hours. Roast at high temperature for 2.5 hours to remove crystal water, add 210.5g of diatomaceous earth to the attapulgite clay for removing crystal water, and mix in a high-speed mixer for 30 minutes to obtain an attapulgite that efficiently removes dioxins from waste incineration waste gas Clay composite adsorbent A. Put the prepared attapulgite clay composite adsorbent A into a fixed-bed reactor, control the reaction temperature at 105°C, and set the gas hourly space velocity at 3000h -1 The ratio of dioxin concentration is 6.3ngTEQ / nm 3 waste incineration flue gas, the concentration of dioxin in the flue gas after adsorption is 0.3ngTEQ / nm 3 .

Embodiment 2

[0021] Weigh 4000.0g of attapulgite clay with a particle size of 3mm to 5mm, add 1600.0g of 30% sulfuric acid aqueous solution, and activate it at a reaction temperature of 100°C for 10 hours. Roast at high temperature for 5.0 hours to remove crystal water, add 1000.0g of diatomaceous earth to the attapulgite clay for removing crystal water, and mix in a high-speed mixer for 10 minutes to obtain an attapulgite that efficiently removes dioxins from waste incineration waste gas Clay composite adsorbent B. Put the prepared attapulgite clay composite adsorbent B into a fixed-bed reactor, control the reaction temperature at 145°C, and set the gas hourly space velocity at 6000h -1 The ratio of dioxin concentration is 2.1ngTEQ / nm 3 waste incineration flue gas, the concentration of dioxin in the flue gas after adsorption is 0.2ngTEQ / nm 3 .

Embodiment 3

[0023] Weigh 4000.0g of attapulgite clay with a particle size of 3mm to 5mm, add 1600.0g of sulfuric acid aqueous solution with a concentration of 60%, and activate it at a reaction temperature of 120°C for 4 hours. Roasting at high temperature for 0.5 hours to remove crystal water, add 210.5g of diatomaceous earth to the attapulgite clay for removal of crystal water, and mix in a high-speed mixer for 30 minutes to obtain an attapulgite that efficiently removes dioxins from waste incineration waste gas Clay composite adsorbent C. The prepared attapulgite clay composite adsorbent C was loaded into a fixed bed reactor, the reaction temperature was controlled at 105 °C, and the gas hourly space velocity was 3000 h -1 The ratio of dioxin concentration is 6.3ngTEQ / nm 3 waste incineration flue gas, the concentration of dioxin in the flue gas after adsorption is 0.3ngTEQ / nm 3 ; The reaction temperature is controlled at 210°C, other conditions remain unchanged, and the concentration...

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Abstract

The invention discloses an attapulgite-clay composite adsorbent and a preparation method thereof. The attapulgite-clay composite adsorbent is applied for removing dioxin in garbage incineration exhaust gas. According to the attapulgite-clay composite adsorbent, cheap attapulgite original soil is adopted as a precursor; an acidification treatment is adopted; and a small amount of diatomite is added in auxiliary. The preparation method is simple. The cost of the absorbent is only 1 / 5 to 1 / 10 of that of active carbon. The absorbent shows good performance in removing dioxin in garbage incineration exhaust gas. The concentration of dioxin in flue gas delivered through an absorption bed layer can be reduced to below 0.3ngTEQ / nm<3>. The attapulgite-clay used for absorbing dioxin can be applied as a construction material, and problems such as environment pollution caused by subsequent releasing of dioxin is prevented. The preparation process is green and friendly. The absorbent has good industrialized application prospect.

Description

1. Technical field [0001] The invention relates to an adsorbent for removing dioxins from waste incineration waste gas, a preparation method and an application thereof, in particular to an attapulgite composite clay for adsorbing and removing dioxins, a preparation method and an application thereof. 2. Background technology [0002] Dioxin is a general term for a class of chlorinated heterocyclic aromatic hydrocarbons present in waste incineration waste gas, with a total of more than 210 homologues and isomers. Such substances are not only stable in nature and need to be decomposed under oxygen-enriched conditions higher than 850°C, but also have super carcinogenic toxicity, reproductive toxicity, endocrine toxicity and immune suppression. Once the dioxins in waste incineration exhaust gas are released into nature, they will continue to accumulate and cause long-lasting harm to humans and the surrounding living environment. At home and abroad, the removal of dioxins in wast...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J20/14B01J20/30B01D53/02
Inventor 马正东刘经伟
Owner 安徽力奥环境新材料有限公司