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Method for preparing acetosyringone from alkali lignin at low temperatures under ethanol conditions

A technology for acetosyringone and alkali lignin, which is applied in the preparation of carbon-based compounds, chemical instruments and methods, preparation of organic compounds, etc., can solve problems such as expensive raw materials, reduce environmental pollution, improve utilization, and expand preparation effect of source

Inactive Publication Date: 2017-04-19
ZHEJIANG SCI-TECH UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Although the two routes can obtain the final product through one-step reaction, the raw materials are expensive

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0012] First, add 0.6 g of alkali lignin sample and 30 mL of absolute ethanol into the SLP miniature high-temperature and high-pressure reactor. Secondly, set the reaction temperature to 135 °C, the reaction time to 4 h, and the pressure when reaching the reaction temperature to 0 MPa. After the reaction was over, the reactor was rapidly cooled to room temperature. Next, a G5 sand core funnel was used for solid-liquid separation, and the solid-phase product was washed with high-performance liquid chromatography-grade isopropanol and tetrahydrofuran until it was colorless. Then, put the solid phase product in a constant temperature drying oven at 50°C and dry it to a constant weight, and weigh it to determine the yield of solid phase residual coke. Finally, the liquid phase product was adjusted to 100 mL with isopropanol, and 40 mL was poured into a disposable plastic petri dish, and dried in a constant temperature drying oven at 50 °C to constant weight.

Embodiment 2

[0014] First, add 0.6 g of alkali lignin sample and 30 mL of absolute ethanol into the SLP miniature high-temperature and high-pressure reactor. Secondly, set the reaction temperature at 150 °C, the reaction time at 4 h, and the pressure at the reaction temperature at 0.8 MPa. After the reaction was over, the reactor was rapidly cooled to room temperature. Next, a G5 sand core funnel was used for solid-liquid separation, and the solid-phase product was washed with high-performance liquid chromatography-grade isopropanol and tetrahydrofuran until it was colorless. Then, put the solid phase product in a constant temperature drying oven at 50°C and dry it to a constant weight, and weigh it to determine the yield of solid phase residual coke. Finally, the liquid phase product was adjusted to 100 mL with isopropanol, and 40 mL was poured into a disposable plastic petri dish, and dried in a constant temperature drying oven at 50 °C to constant weight.

Embodiment 3

[0016] First, add 0.6 g of alkali lignin sample and 30 mL of absolute ethanol into the SLP miniature high-temperature and high-pressure reactor. Secondly, set the reaction temperature at 180 °C, the reaction time at 4 h, and the pressure at the reaction temperature at 3.2 MPa. After the reaction was over, the reactor was rapidly cooled to room temperature. Next, a G5 sand core funnel was used for solid-liquid separation, and the solid-phase product was washed with high-performance liquid chromatography-grade isopropanol and tetrahydrofuran until it was colorless. Then, put the solid phase product in a constant temperature drying oven at 50°C and dry it to a constant weight, and weigh it to determine the yield of solid phase residual coke. Finally, the liquid phase product was adjusted to 100 mL with isopropanol, and 40 mL was poured into a disposable plastic petri dish, and dried in a constant temperature drying oven at 50 °C to constant weight.

[0017] It can be seen from ...

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PUM

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Abstract

The invention relates to a method for preparing acetosyringone from alkali lignin at low temperatures under ethanol conditions. The method comprises the steps: preparing lignin, and treating the lignin, so as to obtain the alkali lignin; then, adding an alkali lignin sample and anhydrous ethanol into an SLP miniature high-pressure high-temperature reactor, and carrying out a reaction; and finally, carrying out solid-liquid separation by adopting a sand-core funnel. The method for preparing the acetosyringone from the alkali lignin through depolymerization has the advantages that the depolymerization temperature is relatively low, and the acetosyringone is a main liquid-phase product at low temperatures, particularly 150 DEG C and 180 DEG C, is almost the only liquid-phase product with obvious absorption peaks which can be detected.

Description

technical field [0001] The invention relates to the preparation of bio-based chemicals by thermochemical conversion of lignin, in particular to a method for preparing acetylsyringone at low temperature under the condition of alkali lignin ethanol. [0002] technical background [0003] As human beings pay more and more attention to environmental problems caused by the excessive use of traditional fossil resources, the demand for developing renewable green resources to replace petrochemical products is increasing year by year. According to statistics, about 50 million tons of lignin by-products are produced in pulp and paper industry wastewater every year. However, it is directly discharged into rivers with waste water or burned after being concentrated, which not only causes a huge waste of resources, but also pollutes the environment. Lignin is a phenolic random polymer with a three-dimensional network structure connected by phenylpropane structural units through ether bond...

Claims

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Application Information

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IPC IPC(8): C07C45/00C07C45/51C07C49/84
CPCC07C45/00C07C45/51C07C49/84
Inventor 郭大亮王林芳陈梦薇张维亮张兴枝
Owner ZHEJIANG SCI-TECH UNIV