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A kind of superhydrophobic polyimide foam and preparation method thereof

A water polyimide and foam technology, applied in the field of super-hydrophobic polyimide foam and its preparation, can solve the problems of affecting the use effect, low water absorption, etc., achieves good flame retardancy, excellent hydrophobicity, and is beneficial The effect of industrial production and promotion

Active Publication Date: 2019-03-29
青岛思贤化工科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The water absorption rate of isocyanate-based polyimide foam is already very low, but water can still penetrate into the foam, which will affect its use effect to a certain extent in some special environments

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] (1) According to the number of parts by mass, dissolve 100 parts of pyromellitic dianhydride in 80 parts of polar solvent N, N-dimethylformamide in the reactor, then add 10 parts of ethylene glycol, and heat to 110 ℃ for 1.5 hours, then cooled to room temperature, and then sequentially added 5 parts of hydrogen-containing silicone oil with a hydrogen content of 0.2%, 10 parts of triethylenediamine catalyst, and 5 parts of SiC type polyether modified silicone oil in proportion, and stirred evenly to obtain Foam precursor.

[0018] (2) Stir and mix the prepared foam precursor and 160 parts of polyphenyl polymethyl polyisocyanate with a paddle mixer, pour into a mold for foam molding to obtain a foam intermediate.

[0019] (3) Put the foam intermediate in a microwave oven and heat it for 1 hour to further solidify it. Then the foam was placed in an infrared oven and heated to 250°C, and the finished product was obtained after 2 hours.

[0020] The prepared foam density i...

Embodiment 2

[0022] (1) According to the number of parts by mass, dissolve 100 parts of pyromellitic dianhydride in 80 parts of polar solvent N, N-dimethylformamide in the reactor, then add 10 parts of ethylene glycol, and heat to 110 ℃ for 1.5 hours, then cooled to room temperature, and then sequentially added 30 parts of hydrogen-containing silicone oil with a hydrogen content of 0.2%, 10 parts of triethylenediamine catalyst, and 5 parts of SiC type polyether modified silicone oil in proportion, and stirred evenly to obtain Foam precursor.

[0023] (2) Stir and mix the prepared foam precursor and 160 parts of polyphenyl polymethyl polyisocyanate with a paddle mixer, pour into a mold for foam molding to obtain a foam intermediate.

[0024] (3) Put the foam intermediate in a microwave oven and heat it for 1 hour to further solidify it. Then the foam was placed in an infrared oven and heated to 250°C, and the finished product was obtained after 2 hours.

[0025] The prepared foam density ...

Embodiment 3

[0027] (1) Dissolve 80 parts of 3,3',4,4'-benzophenone tetraacid dianhydride in 20 parts of polar solvent N-methyl-2-pyrrolidone in a reaction kettle by mass parts, Then add 5 parts of ethylene glycol, heat to 110 ° C for 1.5 hours, then cool to room temperature, and then add 40 parts of hydrogen-containing silicone oil with a hydrogen content of 0.8%, 5 parts of triethylenediamine catalyst, and 5 parts of SiC type polyether-modified silicone oil, and stir evenly to obtain a foam precursor.

[0028] (2) Stir and mix the prepared foam precursor and 150 parts of polyphenyl polymethyl polyisocyanate with a paddle mixer, pour into a mold for foam molding to obtain a foam intermediate.

[0029] (3) Put the foam intermediate in a microwave oven and heat it for 1 hour to further solidify it. Then the foam was placed in an infrared oven and heated to 250°C, and the finished product was obtained after 2 hours. The resulting foam density is 15kg / m 3 , with superhydrophobicity, the wa...

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PUM

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Abstract

The invention relates to a super-hydrophobic polyimide foam and a production method thereof, and belongs to the technical field of polymeric materials. The super-hydrophobic polyimide foam comprises, by mass, 80-120 parts of aromatic dianhydride, 20-90 parts of a polar solvent, 5-100 parts of hydrosilicone oil, 5-20 parts of low molecular alcohol, 5-20 parts of polyether modified silicone oil, 5-10 parts of a catalyst and 150-300 parts of polyisocyanate. Compared with polyimide foams in the prior art, the super-hydrophobic polyimide foam has the advantages of excellent hydrophobicity, good heat resistance, good stability and good flame retardation property; and the method has the advantages of simple process flow, and facilitation of industrial production and promotion.

Description

technical field [0001] The invention relates to a superhydrophobic polyimide foam and a preparation method thereof, belonging to the technical field of polymer materials. Background technique [0002] Polyimide foam is widely used in ships, aircraft carriers, submarines, and aircraft as heat and sound insulation materials in the world because of its excellent flame retardancy, heat insulation, sound insulation, low smoke and low toxicity. [0003] Isocyanate-based polyimide foam is a kind of thermosetting polyimide prepared by polycondensation reaction of aromatic dianhydride or aromatic ester in the presence of a catalyst, using the generated low molecular weight, such as carbon dioxide, as a blowing agent Styrofoam. Since free foaming at room temperature is used in the process, and the purity requirements of raw materials are relatively low, it has very obvious advantages in industrial production. [0004] As a heat insulation material, if it absorbs water, it will great...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08G73/10
CPCC08G73/1035C08G73/106
Inventor 宫勋李荣勋其他发明人请求不公开姓名
Owner 青岛思贤化工科技有限公司