A kind of antistatic gas separation composite membrane and preparation method thereof
A gas separation and anti-static technology, applied in separation methods, semi-permeable membrane separation, dispersed particle separation, etc., can solve the problems of complicated production process, difficult to prepare gas separation composite membrane, insoluble and infusible, etc., and achieve wide application foreground effect
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Embodiment 1
[0036] Dissolve 70 parts of vinylmethylsiloxane-octylmethicone-dimethylsiloxane copolymer in 930 parts of isooctane, add 4 parts of polymethylhydrogensiloxane, 3 parts of 1 , 3-divinyl-1,1,3,3-tetramethyldisiloxane platinum complex, stirred at 40°C for 60 minutes, then added 1 part of 1-octyl-3-methylimidazolium tetrafluoroboron salt, stirred at 40°C for 30 minutes, and prepared as a membrane solution for the separation layer. The membrane solution of the separation layer was evenly coated on the polyacrylonitrile bottom membrane with a pore size of 25 nm, dried at room temperature for 10 minutes, and then dried at 100°C for 20 minutes to prepare a composite membrane. Test its O at 25°C 2 and N 2 The permeation and separation properties of the flux are J N2 =0.28m 3 / m 2 h bar, α O2 / N2 =2.33. Test its surface resistance to measure as 10 8 Ω.
Embodiment 2
[0038] Dissolve 70 parts of vinylmethylsiloxane-octylmethicone-dimethylsiloxane copolymer in 930 parts of isooctane, add 4 parts of polymethylhydrogensiloxane, 3 parts of 1 , 3-divinyl-1,1,3,3-tetramethyldisiloxane platinum complex, stirred at 40°C for 60 minutes, then added 10 parts of 1-octyl-3-methylimidazolium tetrafluoroboron acid salt, and continued to stir at 40°C for 60 minutes to prepare a separation layer membrane solution. The membrane solution of the separation layer was evenly coated on the polyacrylonitrile bottom membrane with a pore size of 25 nm, dried at room temperature for 10 minutes, and then dried at 100°C for 20 minutes to prepare a composite membrane. Test its O at 25°C 2 and N 2 The permeation and separation properties of the flux are J N2 =0.24m 3 / m 2 h bar, α O2 / N2 =2.33. Test its surface resistance to measure as 10 6 Ω.
Embodiment 3
[0040] Dissolve 70 parts of vinylmethylsiloxane-octylmethicone-dimethylsiloxane copolymer in 930 parts of isooctane, add 4 parts of polymethylhydrogensiloxane, 3 parts of 1 , 3-divinyl-1,1,3,3-tetramethyldisiloxane platinum complex, add 10 parts of 1-octyl-3-methylimidazolium tetrafluoroborate, stir at 40°C 90min, prepare the separation layer membrane solution. The membrane solution of the separation layer was evenly coated on the polyacrylonitrile bottom membrane with a pore size of 25 nm, dried at room temperature for 10 minutes, and then dried at 100°C for 20 minutes to prepare a composite membrane. Test its O at 25°C2 and N 2 The permeation and separation properties of the flux are J N2 =0.28m 3 / m 2 h bar, α O2 / N2 =2.33. Test its surface resistance to measure as 10 6 Ω.
[0041] In Comparative Example 1, no ionic liquid was added, and the prepared composite membrane had N 2 Flux and O 2 / N 2 The selectivity is J N2 =0.28m 3 / m 2 h bar, α O2 / N2 =2.33. The s...
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