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Polydopamine/manganese dioxide composite membrane and preparation method thereof

A polydopamine and manganese dioxide technology, applied in chemical instruments and methods, membrane technology, semi-permeable membrane separation, etc., can solve the problem of few types of modifiers, achieve low equipment requirements, increase uniform dispersion, and good affinity. The effect of water anti-pollution properties

Inactive Publication Date: 2018-11-20
FUZHOU UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, there are also problems such as fewer types of modifiers for coating

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0020] A kind of preparation method of polydopamine / manganese dioxide composite film, concrete steps are:

[0021] 1) Preparation of polydopamine surface coating film: put dopamine hydrochloride (initial concentration in the mixed solution: 2 mg / L) into 10 mM Tris solution, and set the volume to 200mL to obtain a mixed solution; commercial polydopamine The vinylidene fluoride microfiltration membrane was immersed in the mixed solution, stirred at room temperature for 24 hours, washed with water, placed in a vacuum drying oven, and dried at 30°C to obtain a polydopamine surface-coated membrane, which was then used;

[0022] 2) Preparation of a polydopamine / manganese dioxide composite film: immerse the polydopamine surface-coated film in 20 mL of 0.6 mM potassium permanganate solution and 0.2 mL of 1 M H2SO4 mixed solution, shake at room temperature for 2 minutes, Take it out, wash it with water, and dry it at 50°C to obtain a polydopamine / manganese dioxide composite film.

[0...

Embodiment 2

[0025] A kind of preparation method of polydopamine / manganese dioxide composite film, concrete steps are:

[0026] 1) Preparation of polydopamine surface coating film: put dopamine hydrochloride (initial concentration in the mixed solution: 4 mg / L) into 10 mM Tris solution, and set the volume to 200mL to obtain a mixed solution; commercial polydopamine The vinylidene fluoride microfiltration membrane was immersed in the mixed solution, stirred at room temperature for 24 hours, washed with water, placed in a vacuum drying oven, and dried at 30°C to obtain a polydopamine surface-coated membrane, which was then used;

[0027] 2) Preparation of a polydopamine / manganese dioxide composite membrane: immerse the polydopamine surface-coated membrane in 20 mL of 0.6 mM potassium permanganate solution and 0.3 mL of 1 M H2SO4 mixed solution, and shake at room temperature for 2 minutes , taken out, washed with water, and dried at 50°C to obtain a polydopamine / manganese dioxide composite fi...

Embodiment 3

[0030] A kind of preparation method of polydopamine / manganese dioxide composite film, concrete steps are:

[0031] 1) Preparation of polydopamine surface coating film: put dopamine hydrochloride (initial concentration in the mixed solution: 6 mg / L) into 10 mM Tris solution, and set the volume to 200 mL to obtain a mixed solution; commercial polydopamine The vinylidene fluoride microfiltration membrane was immersed in the mixed solution, stirred at room temperature for 24 hours, washed with water, placed in a vacuum drying oven, and dried at 30°C to obtain a polydopamine surface-coated membrane, which was then used;

[0032] 2) Preparation of a polydopamine / manganese dioxide composite membrane: immerse the polydopamine surface-coated membrane in 20 mL of 0.6 mM potassium permanganate solution and 0.4 mL of 1 M H2SO4 mixed solution, and shake at room temperature for 2 minutes , taken out, washed with water, and dried at 50°C to obtain a polydopamine / manganese dioxide composite f...

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PUM

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Abstract

The invention discloses a polydopamine / manganese dioxide composite membrane and a preparation method thereof, and belongs to the field of polymer modification. The method comprises the following steps: firstly preparing a polydopamine surface-coated polyvinylidene fluoride modified membrane, then soaking the membrane into a mixed solution of potassium permanganate and sulfuric acid, and performingformation in situ of manganese dioxide nanoparticles on the surface of the membrane through oxidation reduction reaction through the membrane and the solution, so as to obtain the polydopamine / manganese dioxide composite membrane. The polydopamine / manganese dioxide composite membrane is green and environmentally friendly in materials, simple in technology, easy to operate, low in requirement on equipment, and easy for industrialization implementation, and has excellent hydrophilic performance and dye degradation performance.

Description

technical field [0001] The invention belongs to the field of polymer modification, and in particular relates to a preparation method of a polydopamine / manganese dioxide composite membrane. Background technique [0002] There are many methods for hydrophilic and functional modification of polyvinylidene fluoride (PVDF) membranes, and surface composite modification is one of the most important methods. At present, surface composite modification is mainly divided into two categories: one is to modify the surface by coating, and the other is to modify the surface by grafting. Compared with surface grafting modification, surface coating modification is simple to operate, no special equipment is required, and the application trend is obvious. However, there are also problems such as fewer types of modifiers for coating. At present, organic-inorganic composite membranes have received more and more attention due to the introduction of hydrophilic and environmentally friendly inorg...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01D71/60B01D71/34B01D71/02B01D69/12B01D67/00
CPCB01D67/0079B01D69/125B01D71/024B01D71/34B01D71/60
Inventor 李建华张德彬郑徽张博鑫倪惺惺张其清
Owner FUZHOU UNIV