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A kind of preparation method of γ-valerolactone/glycerol system high-yield lignin micro-nanospheres

A technology of micro-nanospheres and lignin, which is applied to the preparation of microspheres, microcapsule preparations, etc., can solve the problems of cumbersome preparation process, time-consuming, poor uniformity of lignin micro-nanospheres, etc., and achieves small size, large specific surface area, The effect of good diffusivity

Active Publication Date: 2021-04-30
TIANJIN UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The existing process of preparing colloidal spheres from acetylated lignin inevitably uses organic solvents that are harmful to the environment and the preparation process is cumbersome. Poor and time-consuming

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0011] Weigh a certain amount of alkali lignin, add it into the GVL solution according to the solid-to-liquid ratio of 1:50 (m / v), and stir to dissolve all the lignin. According to the ratio of GVL to glycerin of 1:5, the above solution was added to glycerin to divide into two layers. Raise the temperature to 60°C, GVL and glycerin are miscible, and stir magnetically for 10 minutes. After the reaction, lower the temperature to room temperature, add water to disperse lignin micronanospheres according to the ratio of mixed solvent and water (v / v) of 1:5, and centrifuge at high speed to obtain lignin micronanospheres with uniform particle size.

Embodiment 2

[0013] A certain quality of kraft lignin was weighed and added into the GVL solution according to the solid-liquid ratio of 1:100 (m / v) to dissolve all the lignin. According to the ratio of GVL to glycerol of 1:10, the above solution was added to glycerin and divided into two layers. The temperature was raised to 80°C, GVL was mixed with glycerol, and OP-10 with a mass fraction of 8% relative to lignin was added, and magnetically stirred for 20 minutes. After the reaction, lower the temperature to room temperature, add water to disperse lignin micronanospheres according to the ratio of mixed solvent and water 1:10 (v / v), and centrifuge at high speed to obtain lignin micronanospheres with uniform particle size.

Embodiment 3

[0015] Weigh a certain mass of organic solvent lignin, and add it into the GVL solution according to the solid-liquid ratio of 1:40 (m / v), so that all the lignin is dissolved. According to the ratio of GVL to glycerol of 1:10, the above solution was added to glycerin and divided into two layers. The temperature was raised to 60°C, GVL was mixed with glycerol, and Span 80 with a mass fraction of 5% of lignin was added, and magnetically stirred for 30 minutes. After the reaction, lower the temperature to room temperature, add water to disperse lignin micronanospheres according to the ratio of mixed solvent and water (v / v) of 1:6, and centrifuge at high speed to obtain lignin micronanospheres with uniform particle size.

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Abstract

The invention belongs to the technical field of lignin nanomaterial preparation, and mainly relates to a preparation method of γ-valerolactone / glycerol system lignin micro-nanospheres. Weigh a certain amount of lignin, add it into the GVL solution according to the ratio of solid-liquid ratio 1:10-1:100 (m / v), stir to dissolve all the lignin; 10. Add the above solution to glycerin and divide into two layers; heat up to 60-100°C, GVL and glycerin are miscible, add emulsifier, and stir magnetically for 5-30min; after the reaction, lower the temperature to room temperature; The ratio of 1:2-1:10 (v / v) is added with water to disperse lignin micronanospheres, and centrifuged at high speed to obtain lignin micronanospheres with uniform particle size. The invention utilizes the green solvent γ-valerolactone / glycerol mixed solvent, and the method adopted is simple in operation and short in time, can greatly improve the preparation efficiency and reduce the preparation cost. By controlling the added amount of the emulsifier, the present invention can prepare lignin micro-nanospheres with high yield and controllable size.

Description

【Technical field】 [0001] The invention belongs to the technical field of lignin nanomaterial preparation, and mainly relates to a method for preparing lignin micro-nanospheres with high yield through a green solvent γ-valerolactone / glycerol system. 【Background technique】 [0002] Lignin is one of the most abundant renewable natural resources in the world. However, lignin has not been widely used due to its complex structure and has been considered as a processing residue. The development of renewable lignin resources into micro-nano materials is a new way to realize the high-value utilization of lignin. [0003] Micro-nanoparticles are very valuable materials, and biomass materials have advantages that traditional inorganic materials do not have, such as renewability, biocompatibility, and biodegradability. Lignin is a biomass material that exists in large quantities, and the preparation of lignin into micro-nano particles is also an important means to improve the utilizat...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J13/02
CPCB01J13/02
Inventor 王冠华司传领陈石林
Owner TIANJIN UNIV OF SCI & TECH