Dispersant, dispersoid, resin composition, composite slurry, electrode film, and non-aqueous electrolyte secondary battery
A dispersant and polymer technology, applied in the direction of non-aqueous electrolyte battery electrodes, secondary batteries, conductive materials dispersed in non-conductive inorganic materials, etc., can solve the problem of not showing the dispersion effect and achieve excellent rate characteristics and cycle characteristics, excellent dispersibility and storage stability, and excellent adhesion and conductivity
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[0182] Hereinafter, the present invention will be described in more detail, but the present invention is not limited to these examples. In the examples, "carbon nanotube" is sometimes abbreviated as "CNT". In addition, "mass %" is described as "%". The compounding quantity in a table|surface is mass %.
[0183] [Example Group α]
[0184] The molecular weight of the dispersant of the present invention, the binder resin, and various physical properties of the dispersion using the dispersant of the present invention were evaluated as follows.
[0185] (Measuring method of weight average molecular weight (Mw))
[0186] The weight average molecular weight (Mw) is determined by gel permeation chromatography (GPC) equipped with a refractive index (Refractive index, RI) detector.
[0187] The device uses HLC-8320GPC (manufactured by Tosoh Corporation), and three separation columns are connected in series, and the packing agent is sequentially used "TSK-GELSUPER (TSK-GELSUPER) AW-400...
Embodiment 98
[0352] According to the composition and dispersion time shown in Table 5β, put 0.8 parts of dispersant, 0.2 parts of additives and 97 parts of dispersion medium into glass bottles (M-225, manufactured by Baiyang Glass Co., Ltd.), fully mix and dissolve or mix, and use as Two parts of CNT were added to the conductive material, and zirconia beads (bead diameter: 0.5mmφ) were used as the medium to disperse with a coating conditioner to obtain a CNT dispersion (CNT dispersion 1β). As shown in Table 5β, CNT dispersion 1β has low viscosity and good storage stability.
[0353] (Example 99β to Example 123β, Comparative Example 18β to Comparative Example 21β)
[0354] According to the composition and dispersion time shown in Table 5β, each CNT dispersion (CNT dispersion 2β to CNT dispersion 26β, comparative CNT dispersion 1β to comparative CNT dispersion 4β) was obtained in the same manner as in Example 100β. As shown in Table 5β, the CNT dispersions of the present invention (CNT disp...
Embodiment 124
[0379] At 150cm in capacity 3 After adding the CNT dispersion (CNT dispersion 1β), CMC and water in the plastic container, use the self-rotating revolution mixer (the defoaming and stirring Taro manufactured by Xinji (Thinky) Company, ARE-310), stir with 2000rpm for 30 seconds, A CNT-containing resin composition 1β was obtained. Then, the active material was added, and the mixture was stirred at 2000 rpm for 150 seconds using the self-rotating mixer. Further, SBR was then added, and stirred at 2000 rpm for 30 seconds using the above-mentioned rotary-revolving mixer, to obtain composite material composition 1β for negative electrode. The nonvolatile content of composite material composition 1β for negative electrodes was 48% by mass. The active material: CNT: CMC: SBR non-volatile component ratio in the composite material composition for negative electrodes was 97:0.5:1:1.5.
[0380] ・Artificial graphite: CGB-20 (manufactured by Nippon Graphite Industry Co., Ltd.), 100% non-...
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