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Ninhydrin functionalized chitosan adsorbent as well as preparation method and application thereof

A technology of ninhydrin hydrate and chitosan, which is applied in chemical instruments and methods, adsorption water/sewage treatment, water pollutants, etc., can solve the problems of reducing adsorption capacity, and achieve easy separation, low cost and high performance Effect

Pending Publication Date: 2021-11-12
KUNMING UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, cross-linking reactions that occur on amino or hydroxyl groups usually reduce the adsorption capacity

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] The ninhydrin functionalized chitosan adsorbent has a structural formula of:

[0023] .

[0024] The preparation method of this ninhydrin functionalized chitosan adsorbent, its concrete steps are as follows:

[0025] Step 1. Dissolve 3.22g of chitosan in 100mL of 2wt% glacial acetic acid and stir until the solution becomes clear, dissolve 1.78g of ninhydrin in 50mL of absolute ethanol, pour the ninhydrin solution into chitosan In the solution, the mixed solution was stirred at 50°C for 18 hours; the ratio of chitosan, ninhydrin, glacial acetic acid and absolute ethanol was 3.22:1.78:100:50g:g:mL:mL;

[0026] Step 2. Add 1 mL of glutaraldehyde solution dropwise to the solution obtained in step 1 as a cross-linking agent. After stirring for 18 hours, add 0.1 mol / L NaOH solution dropwise until the pH of the solution reaches 12. Filter the resulting precipitate and wash until neutral. After drying in a vacuum oven, the solid was ground into a fine powder to obtain a nin...

Embodiment 2

[0030] The ninhydrin functionalized chitosan adsorbent has a structural formula of:

[0031] .

[0032] The preparation method of this ninhydrin functionalized chitosan adsorbent, its concrete steps are as follows:

[0033] Step 1. Dissolve 3.22g of chitosan in 150mL of 2% glacial acetic acid and stir until the solution becomes clear, dissolve 1.78g of ninhydrin in 70mL of absolute ethanol, pour the ninhydrin solution into chitosan In the solution, the mixed solution was stirred at 70°C for 24 hours; the ratio of chitosan, ninhydrin, glacial acetic acid and absolute ethanol was 3.22:1.78:150:70 g:g:mL:mL;

[0034] Step 2. Add 3 mL of glutaraldehyde solution dropwise to the solution obtained in step 1 as a cross-linking agent. After stirring for 24 hours, add 0.1 mol / L NaOH solution dropwise until the pH of the solution reaches 12, filter the resulting precipitate and wash to neutrality. After drying in a vacuum oven, the solid was ground into a fine powder to obtain a ninh...

Embodiment 3

[0038] The ninhydrin functionalized chitosan adsorbent has a structural formula of:

[0039] .

[0040] The preparation method of this ninhydrin functionalized chitosan adsorbent, its concrete steps are as follows:

[0041] Step 1. Dissolve 3.22g of chitosan in 125mL of 2% glacial acetic acid and stir until the solution becomes clear, dissolve 1.78g of ninhydrin in 60mL of absolute ethanol, pour the ninhydrin solution into chitosan In the solution, the mixed solution was stirred at 60°C for 21 hours; the ratio of chitosan, ninhydrin, glacial acetic acid and absolute ethanol was 3.22:1.78:125:60g:g:mL:mL;

[0042] Step 2. Add 2 mL of glutaraldehyde solution dropwise to the solution obtained in step 1 as a cross-linking agent. After stirring for 21 hours, add 0.1 mol / L NaOH solution dropwise until the pH of the solution reaches 12. Filter the precipitate and wash to neutrality. After drying in a vacuum oven, the solid was ground into a fine powder to obtain a ninhydrin funct...

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PUM

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Abstract

The invention relates to a ninhydrin functionalized chitosan adsorbent as well as a preparation method and application thereof, and belongs to the technical field of composite material preparation. The preparation method comprises the following steps: dissolving chitosan in glacial acetic acid, stirring until the solution becomes clear, dissolving ninhydrin in absolute ethyl alcohol, pouring the ninhydrin solution into the chitosan solution, and reacting at a certain temperature; then adding a glutaraldehyde solution to crosslink the chitosan, and dropwise adding a 0.1 mol / L NaOH solution until the pH value of the solution reaches 12; filtering the obtained precipitate and washing to be neutral. and drying in a vacuum oven, and grinding the solid into fine powder to obtain the ninhydrin functionalized chitosan adsorbent. The composite material adsorbent prepared by the method is mainly used for adsorbing and recovering lead ions from a solution.

Description

technical field [0001] The invention relates to a ninhydrin functionalized chitosan adsorbent, a preparation method and an application thereof, belonging to the technical field of composite material preparation. Background technique [0002] Lead is widely used in industries such as metal surface treatment and electrolysis. The pollution of lead to the ecological environment and the harm to public health have become a very serious problem. Due to its resistance to degradation, it can be transferred through the food chain and accumulate in organisms, posing a huge threat to ecosystems and human health. A variety of techniques for the removal of heavy metal ions have been developed, including biological treatment, extraction, ion exchange, precipitation, and adsorption. Most of the above methods are costly and easily cause secondary pollution. The adsorption method has the advantages of good effect, simple operation, economy, and no secondary pollution. It is considered to b...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J20/26B01J20/30C02F1/28C02F101/20
CPCB01J20/26C02F1/285C02F2101/20
Inventor 王仕兴陈应毕唐嘉莉
Owner KUNMING UNIV OF SCI & TECH