Branched polycarbonate produced by reactive extrusion
A technology of polycarbonate resin and reaction, applied in the field of reaction extrusion to prepare branched polycarbonate, which can solve the problems of time-consuming and expensive
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[0069] The preparation of the compositions of the present invention may be accomplished using any of the known blending operations employed for blending thermoplastics, for example blending in a kneader such as a Banbury mixer. Blending can be performed continuously or batchwise.
[0070] After melt extrusion, branching and crosslinking reactions occur in the polycarbonate resin melt.
[0071] The minimum temperature of the melt extrusion reaction should be high enough to generate a melt of the reactants. Such temperatures are achieved in an extruder, or molding machine such as an injection or compression molding machine commonly used for extrusion or molding of polycarbonate.
example 1
[0079] Provide a quantity of linear polycarbonate resin selected from one of the following:
[0080] A. PC135 line type, M w 35000g / mol (main part), or
[0081] B.PC605 linear, soft segment copolymerization-polycarbonate, comprising 10mol% dodecanedioic acid (C 10 Aliphatic series, more sensitive to free radicals).
[0082] As a comparative example, a third resin (branched resin C.PC195) was provided.
[0083] The reference branched resin C.PC195 was supplied by General Electric Company (Pittsfield, MA). This particular resin was prepared directly by synthesis and contained 0.3 mol% tris(4-hydroxyphenyl)ethane as branching agent. This material is mixed in the melting extruder (corotating twin-screw extruder, machine barrel length 950mm, screw rod length 951mm), and mixing condition is, the vacuum degree of 0.5 atmospheric pressure; Rotating speed, 300RPM; Temperature curve from 200 to 300°C.
[0084] Resin A was mixed under the same mixing conditions as described for Re...
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