Polysiloxane compound, preparation method of polysiloxane compound, solidified film of display element and formation method of solidified film
A polysiloxane and display element technology, which is applied in the photoengraving process, static indicator, coating and other directions of the pattern surface, can solve the problem of difficult to form contact holes, etc., and achieves the improvement of adhesion and sufficient resolution. Effect
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[0195] The following synthesis examples and examples are given to describe the present invention more specifically, but the present invention is not limited to the following examples.
[0196] The number average molecular weight (Mn) and weight average molecular weight (Mw) of the hydrolyzed condensate of the hydrolyzable silane compound obtained by each synthesis example below were measured by the gel permeation chromatography (GPC) as follows.
[0197] Device: GPC-101 (manufactured by Showa Denko Co., Ltd.)
[0198] Column: GPC-KF-801, GPC-KF-802, GPC-KF-803, and GPC-KF-804 (manufactured by Showa Denko Co., Ltd.) connected together
[0199] Mobile phase: tetrahydrofuran
[0200] [A] Synthesis example of component polysiloxane
Synthetic example 1
[0202] In a container equipped with a stirrer, add 24 parts by mass of propylene glycol monomethyl ether, then add 39 parts by mass of methyltrimethoxysilane (MTMS), 18 parts by mass of 3-methacryloxypropyltrimethoxy Silane (MPTMS), heated to a solution temperature of 60°C. After the solution temperature reached 60° C., 0.1 parts by mass of formic acid and 19 parts by mass of ion-exchanged water were added, heated to 75° C., and kept for 2 hours. After cooling to 45°C, 28 parts by mass of methyl o-formate was added as a dehydrating agent, followed by stirring for 1 hour. Further, the temperature of the solution was set at 40° C., and the solution was evaporated while maintaining the temperature, thereby removing ion-exchanged water and methanol generated by hydrolytic condensation. Polysiloxane (A-1) was obtained by the above operation. The polysiloxane (A-1) had a solid content concentration of 35% by mass, a weight average molecular weight (Mw) of 1800, and a degree of dis...
Synthetic example 2
[0204]In a container equipped with a stirrer, add 21 parts by mass of propylene glycol monomethyl ether, then add 55 parts by mass of tetramethoxysilane (TEOS), 16 parts by mass of 3-methacryloxypropyltrimethoxysilane (MPTMS), heated to a solution temperature of 60°C. After the solution temperature reached 60° C., 0.1 parts by mass of formic acid and 23 parts by mass of ion-exchanged water were added, heated to 75° C., and kept for 2 hours. After cooling to 45°C, 33 parts by mass of methyl orthoformate was added as a dehydrating agent, and stirred for 1 hour. Further, the temperature of the solution was set at 40° C., and the solution was evaporated while maintaining the temperature, thereby removing ion-exchanged water, methanol and ethanol produced by hydrolytic condensation. Polysiloxane (A-2) was obtained by the above operation. The polysiloxane (A-2) had a solid content concentration of 33% by mass, a weight average molecular weight (Mw) of 2500, and a degree of dispers...
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