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Modified diatomite with multistage-pore structure and preparation method therefor

A diatomite and multi-level pore technology, which is applied in the field of preparation of modified diatomite, can solve the problems of small control range and single pore structure, and achieve the effect of low cost and fast and convenient operation

Inactive Publication Date: 2015-12-16
JILIN UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Due to the single pore structure of diatomite, when it is used as a material for adsorption, noise reduction and noise reduction, the scope for further regulation of its performance is small

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0020] 1) Take 1 kg of diatomite raw soil (above grade two soil), soak it in 1M hydrochloric acid solution for 1 hour, filter off the hydrochloric acid solution, add water and wash it three times; soak the diatomite raw soil after pickling in 1M sodium hydroxide solution 20 minutes, filter the solution, add water and wash three times; 150 ° C blast drying for 3 hours to obtain diatomite with a silica content of more than 98% as a modified raw material;

[0021] 2) Take 1 kg of the above-mentioned diatomite raw material, stir and disperse it in 10 liters of 10% ethanol, add 100 g of tetraethoxysilane, 13 g of tetramethylammonium hydroxide and 100 g of water, and stir at a constant temperature of 35 ° C for 12 hours;

[0022] 3) The product after the above reaction was centrifuged, washed with water three times, dispersed in a high-purity aqueous solution, adjusted to a pH value of about 8.5, and aged at 90°C for 6 hours;

[0023] 4) After the reaction product is centrifuged, it...

Embodiment 2

[0025] 1. Take 1 kg of diatomite raw soil (above grade 2 soil), soak it in 1M hydrochloric acid solution for 1 hour, filter off the hydrochloric acid solution, add water and wash it three times; soak the diatomite raw soil after pickling in 1M sodium hydroxide solution 20 minutes, filter the solution, add water and wash three times; blow dry at 150°C for 3 hours; obtain diatomite with a silica content of more than 98% as a modified raw material;

[0026] 2. Take 1 kg of the above-mentioned diatomite raw material, stir and disperse it in 10 liters of ethanol, add 100 g of tetraethoxysilane, 10 g of cetyltrimethylammonium bromide, 13 g of tetraethylammonium hydroxide and 100 g of water, 35 ℃ constant temperature stirring reaction for 12 hours;

[0027] 3. Centrifuge the product after the above reaction, wash it with water three times, disperse it in a high-purity aqueous solution, adjust the pH value of the solution to about 8.5, and stir and age at 90°C for 6 hours;

[0028] 4...

Embodiment 3

[0030] 1. Take 1 kg of diatomite raw soil (above grade 2 soil), soak it in 1M hydrochloric acid solution for 1 hour, filter off the hydrochloric acid solution, add water and wash it three times; soak the diatomite raw soil after pickling in 1M sodium hydroxide solution 20 minutes, filter the solution, add water and wash three times; blow dry at 150°C for 3 hours; obtain diatomite with a silica content of more than 98% as a modified raw material;

[0031] 2. Take 1kg of the above-mentioned diatomite raw material, stir and disperse it in 10 liters of ethanol, add 100g of tetraethoxysilane, 10g of cetyltrimethylammonium bromide, 13g of tetrabutylammonium hydroxide and 100g of water, and keep the temperature at 35°C Stirring and reacting for 12 hours;

[0032] 3. Centrifuge the product after the above reaction, wash it with water three times, disperse it in a high-purity aqueous solution, adjust the pH value of the solution to about 8.5, and stir and age at 90°C for 6 hours;

[0...

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PUM

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Abstract

The invention provides modified diatomite with a multistage-pore structure and a preparation method therefor. According to the method, pore passages of diatomite are modified, mesoporous and microporous structures are added into the original macroporous structure of the diatomite, and multistage-pore materials with microporous and mesoporous combination or mesoporous and macroporous combination or microporous and macroporous combination can be obtained specifically. According to the modified diatomite with the multistage-pore structure and the preparation method therefor, the preparation of the multistage-pore materials is realized, and the preparation method is quick and convenient in operation and low in cost.

Description

technical field [0001] The invention belongs to the technical field of diatomite inorganic materials, specifically relates to a modified diatomite with a multi-level pore structure, and further provides a preparation method of the modified diatomite. technical background [0002] Diatomite is a siliceous biosedimentary rock formed by diatoms, the main component of which is porous amorphous SiO 2 , and contains a small amount of Fe 2 o 3 , CaO, MgO, Al 2 o 3 and organic impurities. The biggest characteristic of diatomite material is that it has a porous structure and a small specific gravity. It is commonly used in industry as filter aids, insulation materials, fillers, etc., and has a wide range of applications in many fields such as filtration, resins, coatings, coatings, building materials, and medicine. The pore distribution of diatomite is single, and the pore diameter range is above 500nm, which basically belongs to macroporous material. The pore structure varies...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C01B33/12
Inventor 庄家骐韩延东杨文胜
Owner JILIN UNIV