Novel organic material and application thereof
An organic material and a new type of technology, applied in the field of organic electroluminescence display, which can solve the problems of crystallization, poor film formation, and unstable structure.
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Embodiment 1
[0069] Synthesis of (Compound II-1-4)
[0070] The synthetic route is as follows:
[0071]
[0072] Synthesis of compound II-1-4
[0073] 1 liter three-neck flask, equipped with magnetic stirring, add 40.07g (0.378mol) of sodium carbonate, 58.59g of phenanthrene[9,10-d]thiazol-2-ylboronic acid (purity 99%, 0.21mol) and 100ml of toluene in sequence after nitrogen replacement . After nitrogen replacement again, 0.5 g of Pd132 was added in sequence. After the addition, the temperature was raised to 80°C. Start to drop a solution consisting of 44 g of compound P1 (purity 99%, 0.1 mol) and 100 ml of toluene, and control the temperature at 75-90°C. Cool down to room temperature, add 100ml of deionized water for hydrolysis, stir for 10 minutes, filter, filter cake washed several times with DMF, and filter to obtain 60.36g of light yellow solid with a purity of 99% and a yield of 79%.
[0074] Product MS (m / e): 523; Elemental analysis (C 50 h 24 N 2 o 2 S 2 ): theoretic...
Embodiment 2
[0076] Synthesis of (Compound II-1-7)
[0077] The synthetic route is as follows:
[0078]
[0079] Synthesis of compound II-1-7
[0080] 1 liter three-neck flask, equipped with magnetic stirring, after nitrogen replacement, add sodium carbonate 40.07g (0.378mol), (4-(1-phenyl-1H-benzo[d]imidazol-2-yl)phenyl)boronic acid 65.94 g (purity 99%, 0.21mol) and toluene 100ml. After nitrogen replacement again, 0.5 g of Pd132 was added in sequence. After the addition, the temperature was raised to 80°C. Start to drop a solution consisting of 44 g of compound P1 (purity 99%, 0.1 mol) and 100 ml of toluene, and control the temperature at 75-90°C. Cool down to room temperature, add 100ml of deionized water for hydrolysis, stir for 10 minutes, filter, filter the cake with DMF and wash it several times, and filter to obtain 66.26g of a light yellow solid with a purity of 99% and a yield of 81%.
[0081] Product MS (m / e): 818; Elemental Analysis (C 58 h 34 N 4 o 2 ): theoretica...
Embodiment 3
[0083] Synthesis of (Compound II-1-12)
[0084] The synthetic route is as follows:
[0085]
[0086] Synthesis of compound II-1-12
[0087] A 1-liter three-neck flask equipped with magnetic stirring, 40.07 g (0.378 mol) of sodium carbonate, 17.93 g of benzo[d]oxazol-2-ylboronic acid (99% purity, 0.11 mol) and 100 ml of toluene were sequentially added after nitrogen replacement. After nitrogen replacement again, 0.5g of Pd132 was added in sequence. After the addition, the temperature was raised to 80°C. Start to drop a solution consisting of 44 g of compound P1 (purity 99%, 0.1 mol) and 100 ml of toluene, and control the temperature at 75-90°C. Cool down to room temperature, add 100ml of deionized water to hydrolyze, stir for 10 minutes, filter, filter cake is repeatedly boiled and washed with DMF several times, and filter to obtain 31.52g of light yellow solid with a purity of 99% and a yield of 79%.
[0088] Product MS (m / e): 399; elemental analysis (C 27 h 13 NO ...
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