Amphiphilic biodegradable TPU film and preparation method thereof
A biodegradable and amphiphilic technology, applied in the field of polyurethane, can solve the problems affecting the normal use of the film, lack of amphiphilicity, and poor biodegradability of TPU materials, and achieve the effect of improving amphiphilicity and biodegradability.
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preparation example 1
[0049] This preparation example provides a kind of preparation method of modified polylactic acid, comprises the steps:
[0050] (1) The diatom frustules are ball milled with a planetary ball mill, the ball milling time is 10 hours, and the ball milling speed is 500r / min. After ball milling, the diatom frustules are placed in a vacuum oven and dried at 60°C for 24 hours;
[0051] (2) Place polylactic acid (number-average molecular weight 40,000) in a vacuum oven at 60°C and dry for 24 hours, then in parts by weight, 90 parts of polylactic acid, 10 parts of pretreated diatom frustules, toughening agent ( 10 parts of acetyl butyl citrate) and 3 parts of plasticizer (epoxidized soybean oil) are mixed and placed in an internal mixer for mixing. The temperature is 180 ° C, the rotating speed is 60 r / min, and the time is 15 minutes to obtain the modified polylactic acid.
[0052] Wherein, the preparation method of diatom frustules refers to the method in the literature (Wang, J.K.;...
preparation example 2
[0054] This preparation example provides a kind of preparation method of modified polylactic acid, comprises the steps:
[0055] (1) The diatom frustules are ball milled with a planetary ball mill, the ball milling time is 5 hours, and the ball milling speed is 1000r / min, after ball milling, the diatom frustules are placed in a vacuum oven and dried at 70°C for 18 hours;
[0056] (2) Place polylactic acid (number-average molecular weight 50000) in a vacuum oven and dry at 70°C for 12 hours, then in parts by weight, 85 parts of polylactic acid, 15 parts of pretreated diatom frustules, toughening agent ( 15 parts of polyethylene glycol 600) and 4 parts of plasticizer (dioctyl phthalate) were mixed and placed in an internal mixer for mixing at a temperature of 185°C, a speed of 50 r / min, and a time of 10 minutes. Modified polylactic acid is obtained.
preparation example 3
[0058] This preparation example provides a kind of preparation method of modified polylactic acid, comprises the steps:
[0059] (1) The diatom frustules are ball-milled with a planetary ball mill, the ball milling time is 12 hours, and the ball milling speed is 300r / min. After the ball milling, the diatom frustules are placed in a vacuum oven and dried at 50°C for 48 hours;
[0060] (2) Place polylactic acid (number-average molecular weight 45,000) in a vacuum oven at 50°C and dry for 48 hours, then in parts by weight, 95 parts of polylactic acid, 5 parts of pretreated diatom frustules, toughening agent ( 2 parts of polycaprolactone) and 1 part of plasticizer (tributyl citrate) are mixed and placed in an internal mixer for kneading. The temperature is 170 ° C, the speed is 80 r / min, and the time is 20 minutes to obtain the modified polylactic acid.
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