Preparation method of coconut oil fatty acid complex ester
A technology of coconut oil fatty acid and complex ester, which is applied in chemical instruments and methods, petroleum industry, lubricating compositions, etc., can solve problems such as inability to obtain a wide viscosity range, insufficient oxidation stability, and unsatisfactory low-temperature performance. The tuning method is simple and easy to control, good thermal and oxidation stability, and good low temperature performance
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[0028] The invention provides a kind of preparation method of coconut oil fatty acid complex ester, comprises the following steps:
[0029] a) reacting neopentyl polyols and dibasic fatty acids for the first time under the action of a solid catalyst to obtain oligomers;
[0030] b) reacting the oligomer obtained in step a) and coconut oil fatty acid for a second time under the action of a silica gel-supported catalyst to obtain a coconut oil fatty acid complex ester.
[0031] In the invention, neopentyl polyol and dibasic fatty acid are reacted for the first time under the action of solid catalyst to obtain oligomer.
[0032] In the present invention, the neopentyl polyol is preferably selected from neopentyl glycol, 2-methyl-2-ethyl-1,3-propanediol, 2,2-diethyl-1,3-propanediol, One or more of 2-methyl-2-propyl-1,3-propanediol, trimethylolethane and trimethylolpropane, more preferably 2-methyl-2-ethyl-1 ,3-propanediol. The present invention has no special limitation on the so...
Embodiment 1
[0083] (1) Take 35.5g (0.3mol) of 2-methyl-2-ethyl-1,3-propanediol, 14.6g (0.1mol) of adipic acid and 20mL of toluene into a 250mL three-necked flask, stir to dissolve with slight heat , then add 2.5g solid catalyst Al 2 (SO 4 ) 3 / Ti(SO 4 ) 2 , heated and stirred in an oil bath at 130°C, refluxed for water separation for 4.0h, filtered to separate the catalyst, and the filtrate was saturated with Na 2 CO 3 After washing with aqueous solution, wash with deionized water until pH ≈ 7. The oil layer was evaporated under reduced pressure at 60°C / 0.09 MPa to obtain oligomers (m=1.1) without the smell of toluene.
[0084] (2) Take 34.0g of the oligomer produced in step (1), 82.6g of coconut oil fatty acid, and 50mL of water-carrying agent toluene and add them to a 300mL three-necked flask, stir evenly, and then add 4.7g of silica gel to carry Al 2 (SO 4 ) 3 / Ti(SO 4 ) 2 Catalyst, heated and stirred in an oil bath at 130°C, refluxed and separated from water for 5.0h, then f...
Embodiment 2
[0086] (1) Take 23.6g (0.2mol) of 2-methyl-2-ethyl-1,3-propanediol, 14.6g (0.1mol) of adipic acid and 20mL of toluene into a 250mL three-necked flask, and stir to dissolve , then add 1.9g solid catalyst Al 2 (SO 4 ) 3 / Ti(SO 4 ) 2 , heated and stirred in an oil bath at 130°C, refluxed for water separation for 4.0h, filtered to separate the catalyst, and the filtrate was saturated with Na 2 CO 3 After washing with aqueous solution, wash with deionized water until pH ≈ 7. The oil layer was evaporated under reduced pressure at 60°C / 0.09 MPa to obtain oligomers (m=2.1) without the smell of toluene.
[0087] (2) Take 55.5g of the oligomer produced in step (1), 82.6g of coconut oil fatty acid, and 60mL of water-carrying agent toluene and add them to a 400mL three-necked flask, stir evenly, and then add 5.5g of silica gel to carry Al 2 (SO 4 ) 3 / Ti(SO 4 ) 2 Catalyst, heated and stirred in an oil bath at 130°C, refluxed and separated from water for 5.0h, then filtered to se...
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