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Method for preparing hydrogen-preparing hydrogen-storing integrated electrode

An electrode and hydrogen storage technology, applied in the direction of electrodes, electrolysis process, electrolysis components, etc., can solve the problems that need to be further improved, and achieve the effects of improving current efficiency, suppressing hydrogen evolution, and increasing speed

Active Publication Date: 2010-04-14
BC P INC CHINA NAT PETROLEUM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] The electrode commonly used in the above hydrogen production and hydrogen storage coupling technology is a composite electrode combined with an organic hydrogenation electrocatalyst and an ion exchange membrane. The electrode selectivity and current efficiency need to be further improved. In order to suppress hydrogen evolution, increase the speed of the main reaction, and improve Current efficiency needs to be improved

Method used

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Examples

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Effect test

preparation example Construction

[0014] The preparation method of the electrode used in the present invention is a step-by-step method for preparing alloy electrodes. Firstly, the ion-exchange membrane is plated with silver by the dipping reduction method, and then the silver amalgam is formed by the chemical deposition method or the dipping reduction method.

[0015] The silver-plating process on the ion-exchange membrane by the immersion reduction method is as follows: prepare a certain concentration of silver ammonium complex salt solution and a certain concentration of formaldehyde solution; assemble the selected ion membrane in the reactor, put the preheated silver ammonium Add the complex salt solution into the reactor to impregnate the metal complex salt oxidant on the surface of the membrane at a constant temperature; after the impregnation, pour out the solution, rinse the inner surface of the reactor with deionized water, and then pour the preheated formaldehyde solution into the reaction After the ...

Embodiment 1

[0029] Plating silver on ion exchange membrane by immersion reduction method: prepare silver ammonium complex salt solution [Ag(NH 3 ) 2 ] + The concentration is 0.01mol / L, and 1% formaldehyde solution; the weighed Nafion membrane is assembled in the reactor, the preheated metal complex salt solution is added to the reactor, the temperature is controlled at 60°C, and ultrasonic constant temperature impregnation For about 40 minutes, the metal complex salt oxidant is impregnated on the surface of the membrane; after the impregnation, pour out the solution, rinse the inner surface of the reactor with deionized water, and pour the formaldehyde solution preheated to 60°C into the reactor for reduction. The reduction reaction time is 1.0 hour; after the reduction is completed, the membrane is taken out from the reactor to be washed, dried, weighed and stored in sequence.

[0030] Preparation of silver amalgam by chemical deposition method: Prepare the silver-plated ion exchange m...

Embodiment 2

[0034] Adopt the dipping reduction method identical with embodiment 1 to silver-plate on ion-exchange membrane: take another condition to be: silver ammonium complex salt solution [Ag(NH 3 ) 2 ] + The concentration is 0.015mol / L, 0.8% formaldehyde solution; the temperature of the reactor is controlled at 50°C, and the ultrasonic constant temperature is immersed for about 40 minutes. The formaldehyde solution preheated to 50°C is poured into the reactor for reduction, and the reduction reaction time is 0.5 hours.

[0035] Preparation of silver amalgam electrode by impregnation reduction method: prepare a certain concentration of HgCl 2 solution and SnCl 2 solution; assemble the selected ionic membrane in the reactor, put the preheated HgCl 2 The solution was added into the reactor and impregnated at a constant temperature; after the impregnation, the solution was poured out, and after the inner surface of the reactor was slightly rinsed with deionized water, the preheated Sn...

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Abstract

The invention relates to a hydrogen making, hydrogen storing combination electrode method of preparation which is applied to electrolyzed water hydrogen making and organic electrocatalysis hydrogen storing technologies. In the invention, the electrocatalyst silver amalgam is plated on the ion exchange membrane based on the multiple step chemical method and combined with the ion exchange membrane,forming a composite electrode, wherein the multiple step chemical method is that the ion exchange membrane is plated with the silver based on the impregnation reduction method and combined with the silver based on the chemical deposit method or the impregnation reduction method, forming the silver amalgam. The process of the electrolyzed water hydrogen making and the organic hydrogenation storing,in which the electrode of the invention is adopted, makes use of mild conditions under which the silver and the mercury are alloyed, the hydrogen overvoltage of the mercury is relatively high, thereby well restricting the hydrogen evolution and improving the reaction velocity, along with easy preparation; moreover, the current efficiency of the alloy electrode prepared based on the method of theinvention reaches 30 to 40 percent and is obviously improved.

Description

technical field [0001] The invention relates to a preparation method of an integrated electrode for hydrogen production and hydrogen storage, which can be applied in the technologies of hydrogen production by electrolysis of water and electrocatalytic hydrogen storage of organic matter. Background technique [0002] Hydrogen energy is considered to be the most potential, pollution-free and environmentally friendly green energy in the new century because of its cleanness, high efficiency and abundance. Various researches on the development and utilization of hydrogen energy have been valued by the industry. The development and utilization of hydrogen energy is based on the storage of hydrogen energy. Combining water electrolysis hydrogen production and organic matter electrocatalytic hydrogen storage as a whole, using ion exchange membrane electrodes through electrochemical process, in the electrochemical process, the electrolysis reaction of water occurs at the anode, so th...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C25B11/00C25B9/10C25B9/23
Inventor 黄海燕俞英
Owner BC P INC CHINA NAT PETROLEUM CORP