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Method for producing phenolic resin adhesive

The technology of a phenolic resin and a production method is applied in the directions of adhesives, aldehyde/ketone condensation polymer adhesives, adhesive types, etc., which can solve the problems of cumbersome processes, reduction of large-scale production, unfavorable production costs and the like, and achieves a simple process. , the effect of low cost

Inactive Publication Date: 2011-03-23
BEIJING UNIV OF CHEM TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] However, the above methods all adopt two-step or multi-step feeding method, and there are multiple heating and cooling operations, and the process is cumbersome, which is not conducive to the further reduction of production cost and large-scale production.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] 1) mixing phenol with wood tar to obtain wood tar-containing phenol, and the mass percentage of wood tar in the wood tar-containing phenol is 10%;

[0018] 2) phenol containing wood tar, formaldehyde and catalyst (5% NaOH aqueous solution) are prepared according to the molar ratio of 1: 1: 0.05;

[0019] 3) Add wood tar-containing phenol and catalyst into the reaction kettle, heat at 35°C for 15 minutes, then raise the temperature to 55°C, and start to add formaldehyde dropwise, and control the drop rate of formaldehyde to complete the dropwise addition within half an hour and maintain the dropping period The temperature of the reaction system is 65°C. After the dropwise addition, heat at 80°C for 2 hours, then add distilled water to adjust the viscosity of the reaction product to 25mpa.s, filter to remove coarse impurities, and finally dehydrate under vacuum at 20°C and 0.098Mpa to obtain Phenolic resin adhesive.

[0020] The solid content of the phenolic resin adhesi...

Embodiment 2

[0022] 1) Heating and distilling wood tar, collecting fractions at 150-250°C, mixing the wood tar fraction with phenol to obtain wood tar-containing phenol, the mass percentage of wood tar fraction in the wood tar-containing phenol is 15%;

[0023] 2) phenol containing wood tar, formaldehyde and catalyst (30% KOH aqueous solution) are prepared according to the molar ratio of 1: 2: 0.3;

[0024] 3) Add wood tar-containing phenol and catalyst into the reaction kettle, heat at 45°C for 20 minutes, then raise the temperature to 65°C, and start to add formaldehyde dropwise, and control the drop rate of formaldehyde to complete the dropwise addition within half an hour and maintain the dropping period The temperature of the reaction system is 70°C. After the dropwise addition, heat at 90°C for 1.5 hours, then add distilled water to adjust the viscosity of the reaction product to 50mpa.s, filter to remove coarse impurities, and finally dehydrate under vacuum at 35°C and 0.09Mpa to obt...

Embodiment 3

[0027] 1) phenol, formaldehyde and catalyst (45% NaOH aqueous solution) are prepared according to the molar ratio of 1: 3: 0.5;

[0028] 2) Add phenol and catalyst to the reaction kettle, heat at 50°C for 30 minutes, then raise the temperature to 70°C, and start adding formaldehyde dropwise, control the drop rate of formaldehyde to complete the dropwise addition within half an hour and maintain the temperature of the reaction system during the dropwise addition After the dropwise addition, heat at 100°C for 1 hour, then add distilled water to adjust the viscosity of the reaction product to 100mpa.s, filter to remove coarse impurities, and finally vacuum dehydrate at 50°C and 0.08Mpa to obtain a phenolic resin adhesive.

[0029] The solid content of the phenolic resin adhesive prepared in Example 3 is 85.0-95.0%, free phenol is less than 5%, free aldehyde is less than 0.1%, pH value is 11-12, viscosity is 6000-9000mPa.s, bonding strength is greater than 1.75MPa, 150°C Under the...

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Abstract

The invention belongs to the field of industrial phenolic resin adhesive for wood. The phenolic resin adhesive is prepared by the following steps of: adding phenol containing wood tar and catalyst into a reaction kettle, heating the mixture for 10 to 30 minutes at the temperature of between 35 and 50 DEG C, heating the mixture to 50 to 70 DEG C, then dripping formaldehyde into the mixture, controlling the formaldehyde dripping rate in half an hour to finish the dripping and keeping the temperature of the reaction system between 60 and 80 DEG C during dripping, heating the mixture for 1 to 3 hours at the temperature of between 80 and 100 DEG C after the dripping is finished, then adding distilled water to adjust the viscosity of the reaction product to between 10 and 100mpa.s, suction filtering the reaction product and removing coarse impurities, and dehydrating the reaction product in vacuum at the temperature of between 20 and 50 DEG C under the condition of 0.08 to 0.098MPa to obtain the phenolic resin adhesive. The method provided by the invention has the advantages of simple process, low cost and high product bonding strength.

Description

technical field [0001] The invention belongs to the field of phenolic resin adhesives for wood industry, and in particular relates to a method for synthesizing phenolic resin adhesives by substituting wood tar for part of phenol. Background technique [0002] Phenolic resin adhesives are widely used in the bonding field of wood-based panels because of their excellent bonding strength, good water resistance, heat resistance and chemical stability. But the price of phenol, the raw material for producing phenolic resin adhesive, is too high. [0003] As a by-product of biomass pyrolysis gasification reaction, wood tar contains phenol, 2-methylphenol, 4-methylphenol, 2-methoxyphenol, 3,4-dimethylphenol, 2-ethyl Phenolic substances such as phenol. If wood tar is used in the process of synthesizing phenolic resin adhesives, not only can the cost be reduced, but also the harm of wood tar to the environment can be avoided. [0004] For example, Zhou Jianbin and others used bamboo...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C09J161/06
Inventor 张鹏远李林
Owner BEIJING UNIV OF CHEM TECH