A clamp-type zn(ii) metal-organic complex, its preparation method and its application in visual recognition of adenosine triphosphate
A metal-organic and complex technology, which is applied in the direction of zinc-organic compounds, through chemical reaction of materials, and material analysis through observation of the influence of chemical indicators, can solve problems that are not simple, direct, fast, and effective. Accurate identification of adenosine triphosphate, cumbersome detection steps and other issues
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Embodiment 1
[0021] Example 1: Preparation of pincer Zn (II) metal organic complex 1:
[0022] In a 250 mL round bottom flask, add terpyridine S1 (2.993 g, 10 mmol), zinc nitrate hexahydrate (3.57 g, 12 mmol), and anhydrous methanol, respectively. The reaction was stirred at room temperature for 24 hours. A white solid formed in the reaction system. The white solid was obtained by filtration, washed three times with anhydrous methanol, and dried in vacuo to obtain 3.91 g of the corresponding pincer Zn(II) metal organic complex 1. The yield was 80%.
[0023] High resolution mass spectrometry (HR-MS, ESI): m / z 425.0228 (calcd, [M-NO 3 ] + ); 425.0223(found, [M-NO 3 ] + ).
Embodiment 2
[0024] Example 2: Using pincer-type Zn (II) metal organic complex 1 and 0.25 times the molar equivalent of adenosine triphosphate mixed in water, the conventional operation of the gel preparation after heating and cooling, the formation of two-component metal hydrogel formation to achieve the Naked eye visual recognition of adenosine triphosphate:
[0025] In a 5 mL white sample bottle, add 20 mg pincer-type Zn(II) metal-organic complex 1 and 1 mL water successively, seal it with a polyvinyl fluoride cap, and heat the sample bottle with a heat gun. When the solution inside becomes transparent, that is, the clamp-type Zn(II) metal-organic complex 1 is completely dissolved, the heating is stopped, and the sample bottle is left to stand for a while. It was observed that a white precipitate was formed in the sample bottle, and no metal hydrogel was formed. Add adenosine triphosphate in a molar equivalent of 0.25 times that of the pincer-type Zn(II) metal-organic complex 1 to the ...
Embodiment 3
[0026] Example 3: Using pincer-type Zn(II) metal organic complex 1 and 0.25 times the molar equivalent of adenosine diphosphate mixed in water, the conventional operation of gel preparation after heating and cooling, the situation of forming a precipitate:
[0027] In a 5 mL white sample bottle, add 20 mg pincer-type Zn(II) metal-organic complex 1 and 1 mL water successively, seal it with a polyvinyl fluoride cap, and heat the sample bottle with a heat gun. When the solution inside becomes transparent, that is, the clamp-type Zn(II) metal-organic complex 1 is completely dissolved, the heating is stopped, and the sample bottle is left to stand for a while. It was observed that a white precipitate was formed in the sample bottle, and no metal hydrogel was formed. Add adenosine diphosphate in a molar equivalent of 0.25 times that of the clamp-type Zn(II) metal-organic complex 1 to the sample bottle again, seal it again with a polyvinyl fluoride cap, and heat the sample bottle wit...
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