Cyclocarbonate resin based synthetic resin-fixing system, their preparation and use
A technology of cyclic carbonate and artificial resin, applied in drilling compositions, chemical instruments and methods, polyurea/polyurethane adhesives, etc., can solve problems such as high viscosity and partial crystallization tendency
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Embodiment 1
[0115] Example 1: General Operating Regulations I: Cyclic Carbonate Using 4,4'-Diphenylmethane Dicarbamate Diglycerol Carbonate and Trimethylolpropane Triglycidyl Ether as Reactive Diluents Synthesis of resin:
[0116] In a 250 mL glass flask with reflux condenser and with drying tube, stirrer, dropping funnel and thermometer - in the amounts mentioned in Table 1 (Example 3) - pre-place trimethylolpropane triglycidol ether and glycerol carbonate and heated to 60°C in an oil bath. "PMDI" was slowly added dropwise to the reaction mixture so that the temperature did not exceed 80°C. After complete addition of "PMDI", stirring was continued at 80°C to complete the reaction. The completed reaction was checked by means of FT-IR (no isocyanate groups detectable by IR-spectroscopy).
Embodiment 2
[0117] Example 2: General Procedure II: 4,4'-Diphenylmethane dicarbamate diglycerol carbonate with trimethylolpropane triglycidyl ether and neopentyl glycol diglycidyl ether as reactive Alternative Synthesis of Cyclic Carbonate Resins Example of Diluent-Mixture:
[0118] Trimethylolpropane triglycidyl ether, neopentyl glycol diglycidyl ether and glycerol carbonate were pre-placed in the amounts mentioned in Table 3 (Example 4) in a 120 mL plastic cup with a screw cap. After mixing well, add "PMDI" at room temperature and re-mix to a streak-free appearance. The plastic cup containing the reaction mixture was then stored at 40°C to complete the reaction. The completed reaction was checked by means of FT-IR (no isocyanate groups detectable by IR-spectroscopy).
Embodiment 3
[0119] Embodiment 3: the prescription of carbonate resin I:
[0120] The formula of the resin prepared according to embodiment 1 is:
[0121] name Weigh m [g] weight% trim 57.81 60.00 glycerol carbonate 18.54 19.24 "PMDI" 20.00 20.76
[0122] "PMDI" refers to mixtures of MDI (isocyanate functionality 2) and PMDI (isocyanate functionality 3.2) and / or monofunctional isocyanates (isocyanate functionality 1.0) according to Table 2.
[0123] MDI: diphenylmethane diisocyanate - isomer mixture, molecular weight 250 g / mol, isocyanate - functionality 2 (manufacturer's instructions)
[0124] PMDI: diphenylmethane diisocyanate with isomers and homologues of higher degree of functionality, molecular weight 430 g / mol, isocyanate-functionality 3.2 (manufacturer's instructions)
[0125] p-TSI: p-toluenesulfonyl isocyanate, molecular weight 197.21 g / mol, isocyanate-functionality 1
[0126] Trim: trimethylolpropane triglycidyl ether (technical grade ...
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Abstract
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