Aromatic ring modified organic photovoltaic material and preparation method thereof
A technology of organic photovoltaic materials and aromatic rings, applied in the field of photovoltaic materials, can solve the problems of short battery life, insufficient stability and durability, high body resistance, etc., and achieve long battery life, good durability, and good stability Effect
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Embodiment 1
[0056] The aromatic ring modified organic photovoltaic material is prepared by the following method:
[0057] (1) In DMF solvent, 2mol compound (1) and 4mol POCl 3 React at room temperature for 1.5h to obtain compound (2);
[0058]
[0059] MS (m / z): 199.05;
[0060] (2) Under alkaline conditions, 1.5 mol of compound (3-1) was reacted at 350°C for 8 hours, and intramolecular cyclization was performed to obtain compound (4-1);
[0061]
[0062] MS (m / z): 246.12;
[0063] (3) In the presence of TFA catalyst and DDQ oxidant, 1 mol of compound (2) and 1 mol of compound (4-1) were reacted at room temperature for 8 hours to obtain compound (I-1) and compound (II-1);
[0064]
[0065] MS (m / z): 822.32.
Embodiment 2
[0067]Aromatic ring-modified organic photovoltaic materials, prepared by the following method:
[0068] (1) In DMF solvent, 2mol compound (1) and 6mol POCl 3 React at room temperature for 0.5h to obtain compound (2);
[0069]
[0070] MS (m / z): 199.05;
[0071] (2) Under alkaline conditions, 1.5 mol of compound (3-2) was reacted at 340°C for 12 hours, and intramolecular cyclization was performed to obtain compound (4-2);
[0072]
[0073] MS (m / z): 274.15;
[0074] (3) In the presence of TFA catalyst and DDQ oxidant, 1 mol of compound (2) and 1 mol of compound (4-2) were reacted at room temperature for 12 hours to obtain compound (I-2) and compound (II-2).
[0075]
[0076] MS (m / z): 878.38.
Embodiment 3
[0078] Aromatic ring-modified organic photovoltaic materials, prepared by the following method:
[0079] (1) In DMF solvent, 2mol compound (1) and 5mol POCl 3 React at room temperature for 1 h to obtain compound (2);
[0080]
[0081] MS (m / z): 199.05;
[0082] (2) Under alkaline conditions, 1.5 mol of compound (3-3) was reacted at 345°C for 10 h, and intramolecular cyclization was performed to obtain compound (4-3);
[0083]
[0084] MS (m / z): 154.05;
[0085] (3) In the presence of TFA catalyst and DDQ oxidant, 1.1 mol of compound (2) and 1 mol of compound (4-3) were reacted at room temperature for 10 h to obtain compound (I-3) and compound (II-3).
[0086]
[0087] MS (m / z): 738.23.
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