A kind of organosilicon modified polyester resin and preparation method thereof
A technology for modifying polyester and polyester resin, applied in the field of polymer chemical preparation, which can solve the problems of complex construction and waste, and achieve the effects of suitable machinery, fast preparation speed and simple synthesis process
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Embodiment 1
[0052] A preparation method of organosilicon modified polyester resin, the method includes the following steps:
[0053] (1) Mix 42 parts of polybasic organic acids, 33 parts of polyols, 0.2 parts of catalyst and 28 parts of xylene, and react at 4℃ / min to 170℃ for 50min under the protection of nitrogen. Add 0.2 parts of heat stabilizer to 1 ℃ / min Raise temperature to 230℃ and react for 50min while distilling out water. After cooling to 180℃, add 2 parts polyol and 3 parts xylene, heat up to 220℃ at 1℃ / min to react, and add 5 parts toluene after reaction to obtain polyester resin Solution
[0054] (2) Mix 65 parts of the polyester resin solution obtained in step (1), 14 parts of organosilicon intermediate, 0.2 parts of heat stabilizer, 0.3 parts of catalyst and 4 parts of xylene, and heat up to 170°C for 60 minutes under nitrogen protection Then, the temperature is increased to 185°C to react for 60 minutes, and then the temperature is increased to 200°C to react, and the reaction ...
Embodiment 2
[0062] A preparation method of organosilicon modified polyester resin, the method includes the following steps:
[0063] (1) Mix 46 parts of polybasic organic acids, 36 parts of polyols, 0.3 parts of catalyst and 20 parts of xylene, and react at 4℃ / min to 170℃ for 50min under the protection of nitrogen. Add 0.2 parts of heat stabilizer to 1 ℃ / min Raise temperature to 230℃ and react for 50min while distilling out water. After cooling to 180℃, add 2 parts polyol and 4 parts xylene, then heat up to 220℃ at 1℃ / min to react, and add 5 parts toluene after reaction to obtain polyester resin Solution
[0064] (2) Mix 65 parts of the polyester resin solution obtained in step (1), 18 parts of organosilicon intermediate, 0.2 parts of heat stabilizer, 0.4 parts of catalyst and 6 parts of xylene, and heat up to 170°C for 60 minutes under nitrogen protection Then, the temperature is increased to 185°C to react for 60 minutes, and then the temperature is increased to 200°C to react, and the reac...
Embodiment 3
[0072] A preparation method of organosilicon modified polyester resin, the method includes the following steps:
[0073] (1) Mix 52 parts of polybasic organic acids, 40 parts of polyols, 0.3 parts of catalyst and 20 parts of xylene, and react at 4℃ / min to 170℃ for 50min under the protection of nitrogen, and add 0.2 parts of heat stabilizer to 1 ℃ / min Raise temperature to 230℃ and react for 50min while distilling water out, add 2 parts of polyol and 5 parts of xylene after cooling down to 180℃, heat up to 220℃ at 1℃ / min for reaction, add 5 parts of toluene after reaction to obtain polyester resin Solution
[0074] (2) Mix 65 parts of polyester resin solution obtained in step (1), 22 parts of organosilicon intermediate, 0.2 parts of heat stabilizer, 0.7 parts of catalyst and 8 parts of xylene, and heat to 170°C for 60 minutes under nitrogen protection Then, the temperature is increased to 185°C to react for 60 minutes, and then the temperature is increased to 200°C to react, and the...
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