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A preparation method of carbon source for synthesizing large-scale polycrystalline diamond

A polycrystalline diamond, large-scale technology, applied in chemical instruments and methods, ultra-high pressure processes, graphite and other directions, can solve problems such as inconclusive results, achieve high forming density, reduce pressure and temperature, and reduce losses. Effect

Active Publication Date: 2021-07-13
ZHENGZHOU ZHONGNAN JETE SUPERABRASIVES
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] The transformation mechanism of graphite to diamond under the condition of ultra-high pressure and high temperature has been discussed for decades, and no conclusion has been reached so far.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0021] The invention provides a preparation method of a carbon source for synthesizing large-scale polycrystalline diamond, which specifically comprises the following steps:

[0022] 1) Screen the flake graphite for grain size, and take ≤600 mesh as the sample to be treated;

[0023] 2) Put the sample to be processed obtained in step 1) into a ball mill, add alcohol and mix it into a paste, then add steel balls, and perform ball milling on the ball mill for 8-30 hours;

[0024] 3) After the ball milling is completed, use pure water to flush the ball-milled graphite into the beaker, re-classify the particle size, select ≤5000 mesh and then precipitate;

[0025] 4) Pour off the precipitation clear water, add hydrochloric acid and boil on an electric heating furnace for half an hour, further remove impurities, wash with pure water after natural cooling to neutrality, and dry the precipitate obtained after precipitation in a vacuum drying oven;

[0026] 5) The dried precipitate i...

Embodiment approach

[0028] As an embodiment of the present invention, the purity requirements of the graphite flakes described in step 1) of the preparation method are very high, requiring ≥99.99%, and the graphite flakes of this purity can be purchased from LC(-) of Qingdao Baichuan Graphite Co., Ltd. 325-9999 type flake graphite, the purpose of using high-purity flake graphite is to reduce the impurity content in synthetic polycrystalline diamond and ensure the quality of polycrystalline diamond.

[0029] As an embodiment of the present invention, the mass of the steel balls added in step 2) of the preparation method is 10-20 times the mass of the flake graphite of the sample to be treated. As another embodiment of the present invention, the steel balls have three sizes of 6 mm, 8 mm and 10 mm, and are used in a mixture in a mass ratio of 2:3:5.

[0030] As an embodiment of the present invention, the ball mill used in step 2) of the preparation method is an iron ball mill. The reason for using ...

Embodiment 1

[0034] In this example, the flake graphite was screened by a vibration screening machine for grain size, and 325-400 mesh was selected as the sample to be processed, 100 grams of graphite was taken from it, put into an iron ball mill, and an appropriate amount of alcohol was added to mix it into a paste. Add steel balls whose mass ratio is 10 times the weight of graphite (steel balls are 6mm, 8mm, and 10mm in three sizes and mixed in a mass ratio of 2:3:5), tighten the ball mill jar to start ball milling, ball mill for 8 hours, and then use pure Pour the ball-milled graphite into a beaker with water, re-classify the particle size, select a particle size section below 700 mesh and then precipitate; pour out the precipitated water, add an appropriate amount of hydrochloric acid, boil it on an electric furnace for half an hour, further remove impurities, and cool it naturally After washing with pure water until neutral, the precipitate obtained after precipitation was dried in a v...

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PUM

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Abstract

The invention provides a method for preparing a carbon source for synthesizing large-scale polycrystalline diamond. The method uses flake graphite as a raw material, and obtains a carbon source for synthesizing large-scale polycrystalline diamond through processes such as screening, ball milling, finishing treatment, and grading. The method can obtain a carbon source with uniform particle size and high molding density, and can reduce pressure loss caused by volume collapse during the synthesis process. The degree of graphitization, porosity, ash, resistivity, and crystal structure of the carbon source obtained by the preparation method of the present invention can not only greatly reduce the pressure and temperature required for the synthesis of low-growth, high-quality, large-scale polycrystalline diamond, but also achieve stable conversion , The purpose of saving costs.

Description

technical field [0001] The invention belongs to the technical field of raw and auxiliary materials for the production of superhard materials, and particularly relates to a preparation method of a carbon source for synthesizing large-scale polycrystalline diamond. Background technique [0002] At present, there are two main ways to prepare large-scale polycrystalline diamond under high temperature and high pressure: one is to synthesize diamond from graphite and then sinter it from diamond powder; the other is to directly convert graphite into polycrystalline diamond at one time. The pathway is formed by the direct transformation of graphite under the conditions of ultra-high pressure and high temperature of 14~18GPa and 2300~2600K. The overall performance of the polycrystalline diamond synthesized by the second method is far better than the first one, which is the current and future development direction. Large-scale polycrystalline diamond can be widely used in geology, me...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C01B32/21C01B32/215B01J3/06
CPCB01J3/06
Inventor 张相法张奎薛磊王永凯位星鲁翠莲
Owner ZHENGZHOU ZHONGNAN JETE SUPERABRASIVES