Novel process route for modified fatty acid type PET reagent precursor
A compound and selected technology are applied in the preparation of sulfonic acid esters, the preparation of carboxylic acid esters, and the preparation of carboxylic acids by oxidation, which can solve the problems of unfavorable industrial production of materials, excessively long synthesis routes, etc., and achieve low toxicity and danger of reagents, Simple to use effects
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[0105] Reaction formula
[0106]
[0107] 1. Synthesis of Compound 1
[0108] Into a 1-liter three-neck flask, add magnesium chips and a little iodine, and replace and protect with nitrogen. Then 60 ml of anhydrous THF and a small amount of 6-bromo-1-hexene were added and the temperature was raised to initiate the reaction. After initiation, a solution of 162 g of 6-bromo-1-hexene in tetrahydrofuran was slowly added. After the dropwise addition, continue to stir until the reaction is complete.
[0109] Subsequently, 72 g of nonanal was added, and after the reaction was completed, the reaction was quenched with dilute hydrochloric acid, and extracted with dichloromethane. The organic phases were combined and desolvated and then purified by column chromatography. 68 g of compound 1 was obtained as a pale yellow liquid with a yield of 77%.
[0110] 1 H-NMR (300MHz, CDCl 3 )δ: 0.88(t, 3H), 1.28-1.47(m, 20H), 2.06(m, 2H), 3.58(m, 1H), 4.93(dd, 1H), 5.00(dd, 1H), 5.80(m ,...
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