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Recycling treatment method of waste vanadium catalyst

A waste vanadium catalyst, recovery and treatment technology, applied in chemical instruments and methods, catalyst regeneration/reactivation, physical/chemical process catalysts, etc., can solve the problems of complex treatment process, toxic substance pollution, environmental pollution, etc. High, low disposal cost, environmentally friendly effect

Inactive Publication Date: 2018-11-30
HUNAN SANFENG VANADIUM IND CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The purpose of the present invention is to provide a recovery and treatment method for spent vanadium catalysts, which is used to solve the defects of toxic substance pollution, environmental pollution and complex treatment process in the existing waste vanadium catalyst treatment process

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] The recovery treatment method of the spent vanadium catalyst of the present embodiment, it may further comprise the steps:

[0026] Step A: washing the spent vanadium catalyst with a protective solution containing a diester precipitator and oxalic acid, wherein, in the protective solution, the mass fraction of the diester precipitant is 1.5%, and the oxalic acid is 2.5%.

[0027] Step B: Spin and dry the spent vanadium catalyst to obtain a dried spent vanadium catalyst, wherein the spent vanadium catalyst needs to be dried at 100° C. for 2 hours.

[0028] Step C: Soak the dried spent vanadium catalyst in an oxalic acid solution containing 80% by mass fraction, heat at 40°C, add vanadium pentoxide with a mass fraction of 8% to the above solution, heat the solution to 102°C, and react for 5 hours, Then drain or spin dry to obtain an intermediate product containing spent vanadium catalyst. In this step, the pentavalent vanadium stored in the spent vanadium catalyst is con...

Embodiment 2

[0032] The recovery treatment method of the spent vanadium catalyst of the present embodiment, it may further comprise the steps:

[0033] Step A: Washing the spent vanadium catalyst with a protective solution containing a diester precipitator and oxalic acid, wherein, in the protective solution, the mass fraction of the diester precipitant is 0.5%, and the oxalic acid is 1.5%.

[0034] Step B: Spin and dry the spent vanadium catalyst to obtain a dried spent vanadium catalyst, wherein the spent vanadium catalyst needs to be dried at 100° C. for 2 hours.

[0035] Step C: Soak the dried spent vanadium catalyst in an oxalic acid solution containing 30% by mass fraction, heat at 30°C, add vanadium pentoxide with a mass fraction of 2% to the above solution, heat the solution to 80°C, and react 2-5 hours, and then drained or spin-dried to obtain an intermediate product containing spent vanadium catalyst. In this step, the pentavalent vanadium stored in the spent vanadium catalyst i...

Embodiment 3

[0039] The recovery treatment method of the spent vanadium catalyst of the present embodiment, it may further comprise the steps:

[0040] Step A: washing the spent vanadium catalyst with a protection solution containing a diester precipitator and oxalic acid, wherein, in the protection solution, the mass fraction of the diester precipitator is 1%, and the mass fraction of oxalic acid is 2%.

[0041] Step B: Spin and dry the spent vanadium catalyst to obtain a dried spent vanadium catalyst, wherein the spent vanadium catalyst needs to be dried at 100° C. for 2 hours.

[0042] Step C: Soak the dried spent vanadium catalyst in an oxalic acid solution containing 30-80% by mass fraction, heat at 35°C, add vanadium pentoxide with a mass fraction of 5% to the above solution, heat the solution to 90°C, and react 3 hours, and then drained or spin-dried to obtain an intermediate product containing spent vanadium catalyst. In this step, the pentavalent vanadium stored in the waste vana...

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PUM

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Abstract

The invention discloses a recycling treatment method of a waste vanadium catalyst. The recycling treatment method comprises the following steps: A, washing the waste vanadium catalyst by utilizing a solution containing a diester precipitating resistance agent and oxalic acid; B, drying the waste vanadium catalyst in a spinning and baking manner so as to obtain a dried waste vanadium catalyst; C, soaking the dried waste vanadium catalyst with an oxalic acid solution of which the mass percentage is 30 to 80 percent, performing heating at 30 to 40 DEG C, adding vanadium pentoxide of which the mass percentage is 2 to 8 percent into the solution, heating the solution at 80 to 102 DEG C and performing reaction for 2 to 5 hours to obtain an intermediate product containing the waste vanadium catalyst; D, roasting the intermediate product at 100 to 550 DEG C until gas cannot be exhausted, and then finally obtaining the waste vanadium catalyst containing vanadium pentoxide. According to the recycling treatment method of the waste vanadium catalyst disclosed by the invention, through the effects of reagents such as the diester precipitating resistance agent and the oxalic acid, in the recycling treatment process, generation of polluted gas is avoided, wastes are avoided, environmental protection is achieved, and meanwhile, a recycling ratio of the waste vanadium catalyst is high, and themanufacturing cost is low.

Description

technical field [0001] The invention relates to the technical field of recovery and utilization of waste catalysts, in particular to a method for recovery and treatment of waste vanadium catalysts. Background technique [0002] At present, with the continuous development of the sulfuric acid industry, petrochemical industry, and benzene industry, the consumption of spent vanadium catalysts is also increasing, and spent vanadium catalysts are well-known toxic substances. Many scholars and experts at home and abroad have devoted themselves to the study of new chemical disposal methods for spent vanadium catalysts. Although some technological methods for recycling spent vanadium catalysts have been developed, at the same time, they have laid a theoretical and practical foundation for the recycling of spent vanadium resources. Because the waste vanadium catalyst contains a large amount of sulfur, nitrate, carbon, arsenic and other substances, in the traditional recycling process...

Claims

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Application Information

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IPC IPC(8): B01J23/22B01J23/92B01J38/02B01J38/48B01J38/62B01J38/68
CPCB01J23/22B01J23/92B01J38/02B01J38/48B01J38/62B01J38/68Y02P20/584
Inventor 许小弟田兴江
Owner HUNAN SANFENG VANADIUM IND CO LTD