Static pressure piezochromic material and preparation method thereof
A piezochromic and static pressure technology, applied in the field of materials, can solve the problems of small color changes and the inability to realize the adjustment of visible light bands, and achieve the effect of huge application potential
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Embodiment 1
[0021] Weigh 4.20g (20mmol) of 4,4'-biphenyldicarbaldehyde (II), 5.88g (40mmol) of p-methoxyphenylacetonitrile (III) and 0.27g (5mmol) of sodium methoxide and dissolve them in 30ml of absolute ethanol. The reaction was stirred at room temperature for 10 h, and the reaction was terminated when a large amount of solid particles were precipitated. Then put the reaction system into -20 DEG C refrigerator and let it stand overnight for 12h, then filter, precipitate with methanol rinse (20mL * 3) times, after natural drying, a white powder is obtained, i.e. the target product (I) is 8.4g in total, and the yield is 90.0%. It is piezochromic material. 1 H NMR (500MHz, CDCl 3 ): δ (ppm) 8.00 (d, J = 8.5Hz, 4H), 7.76 (d, J = 8.5Hz, 4H), 7.65 (d, J = 8.5, 4H), 7.49 (s, 2H), 7.00 ( d, J=9Hz, 4H), 3.89(s, 6H); MS m / z: 468.4(M+).
Embodiment 2
[0023] Weigh 4.20g (20mmol) of 4,4'-biphenyldicarbaldehyde (II), 6.03g (41mmol) of p-methoxyphenylacetonitrile (III) and 0.27g (5mmol) of sodium methoxide and dissolve them in 30ml of absolute ethanol. The reaction was stirred at room temperature for 10 h, and the reaction was terminated when a large amount of solid particles were precipitated. Then the reaction system was put into -20 DEG C of refrigerator and left to stand overnight for 12h, then filtered, and the precipitate was rinsed with methanol (20mL × 3) times, and after natural drying, a white powder was obtained, that is, a total of 8.52g of the target product (I), and the yield was 91%. It is piezochromic material.
Embodiment 3
[0025] Weigh 4.20g (20mmol) of 4,4'-biphenyldicarbaldehyde (II), 5.88g (40mmol) of p-methoxyphenylacetonitrile (III) and 0.26g (4.8mmol) of sodium methoxide and dissolve them in 40ml of absolute ethanol . The reaction was stirred at room temperature for 10 h, and the reaction was terminated when a large amount of solid particles were precipitated. Then the reaction system was put into -20 DEG C refrigerator and left to stand overnight for 12h, then filtered, and the precipitate was rinsed with methanol (20mL×3) times, and after natural drying, a white powder was obtained, that is, the target product (I) was 8.18g in total, and the yield was 87.4%. It is piezochromic material.
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