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A method for controllable OH free radical synergistic degradation treatment of wastewater containing polysaccharide polymers

A technology of synergistic degradation and polymer, applied in natural water treatment, filtration treatment, sedimentation treatment, etc., can solve problems such as difficult sinking, large amount of mud, and inability to effectively remove high-viscosity fracturing waste liquid impurities, etc., to achieve improved treatment Efficiency, reduction of treatment links, and improvement of oxidation treatment efficiency

Active Publication Date: 2021-11-12
XI'AN PETROLEUM UNIVERSITY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This method can be used to treat high-viscosity fracturing waste fluid with a viscosity > 5mPa·s, and overcomes the shortcomings of conventional coagulation that cannot effectively remove impurities in high-viscosity fracturing waste fluid, flocs are floating, not easy to sink, and a large amount of mud

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] Taking the treatment of guar gum-based oilfield fracturing waste fluid as an example, its viscosity is 30mpa·s, chromaticity is 200 degrees, COD is 3500mg / L, and suspended solids content is 170mg / L. The specific treatment methods are as follows:

[0027] 1L of ferrous sulfate aqueous solution with mass concentration of 20%, 1.5 mL of sodium hydroxide aqueous solution with mass concentration of 10%, and 2L of sodium hypochlorite aqueous solution with mass concentration of 10.5% were transported to a heating device through a metering pump connected to it. In a tubular reactor, the reaction was heated at 70 °C for 30 s. Then, the obtained reaction solution and 45 L of guar gum-based fracturing flowback fluid were immediately pumped into a reactor with stirring, and the oxidation reaction was stirred for 40 min. After the reaction is completed, it is settled in the sedimentation tank for 20 minutes, and then filtered through a quartz sand filter with a particle size of 0.5 ...

Embodiment 2

[0029] Taking the treatment of oilfield drilling waste fluid containing carboxymethyl cellulose as an example, its viscosity is 180mpa·s, chromaticity is 170 degrees, COD is 1500mg / L, and suspended solids content is 130mg / L. The specific treatment method is as follows:

[0030] 1L of ferrous sulfate aqueous solution with mass concentration of 20%, 2mL of sodium hydroxide aqueous solution with mass concentration of 10%, and 4L of sodium chlorite aqueous solution with mass concentration of 10.5% were respectively transported to a heating system with a metering pump connected to it. In the tubular reactor of the device, the reaction was heated at 60°C for 70s. Then immediately the obtained reaction solution and 70 L of oilfield drilling waste liquid containing carboxymethyl cellulose were pumped into a reactor with stirring, and the oxidation reaction was stirred for 40 minutes. After the reaction is completed, it is settled in the sedimentation tank for 30 minutes, and then filt...

Embodiment 3

[0032] Taking the treatment of fracturing waste fluid containing guar gum as an example, its viscosity is 180mpa·s, chromaticity is 170 degrees, COD is 1500mg / L, and suspended solids content is 130mg / L. The specific treatment methods are as follows:

[0033] 1L of ferrous sulfate aqueous solution with mass concentration of 18%, 1mL of potassium hydroxide aqueous solution with mass concentration of 10.5%, and 3L of sodium chlorite aqueous solution with mass concentration of 12.5% ​​were respectively transported to a heating system with a metering pump connected to it. In the tubular reactor of the device, the reaction was heated at 50 °C for 90 s. Then, the obtained reaction solution and 50 L of guar-containing fracturing waste fluid were immediately pumped into a reactor with stirring, and the oxidation reaction was stirred for 40 min. After the reaction is completed, it is settled in the sedimentation tank for 20 minutes, and then filtered through a quartz sand filter with a pa...

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Abstract

The invention discloses a controllable·OH free radical synergistic degradation method for treating polysaccharide-containing polymer sewage. In this method, firstly, the ferrous ion solution is mixed with lye and oxidant and heated to generate OH free radicals, O free radicals and polymerized iron ions, etc., and then it is mixed with polysaccharide-containing polymer sewage to utilize the generated The OH free radicals and O free radicals with high-efficiency oxidation react with the polysaccharide polymers in the sewage and degrade them, and the polymerized iron ions formed form flocs to purify the suspended solids in the sewage. The treated polysaccharide-containing polymer sewage can be reinjected or re-formulated oilfield working fluid. The invention can quickly and efficiently realize the treatment of polysaccharide-containing polymer sewage, and can recycle the treated sewage.

Description

technical field [0001] The invention belongs to the technical field of oil and gas field operation waste liquid treatment, and in particular relates to a treatment method for polysaccharide polymer-containing sewage. Background technique [0002] In the process of oilfield production, due to the needs of drilling and reservoir stimulation, polysaccharide-containing polymers are often used as drilling fluid additives or fracturing fluid additives. , high COD value characteristics. Since the polysaccharide polymers contained in this kind of sewage are easily affected by microorganisms, they will deteriorate and stink, so their treatment and reuse are one of the important contents of oilfield environmental protection work. In order to realize the resourceful and harmless treatment of this kind of wastewater, scientific and technological workers began to use the gel breaking / flocculation composite treatment technology to treat the wastewater in the 1990s. [0003] CN 105540964...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C02F9/04C02F103/38
CPCC02F9/00C02F1/72C02F2305/023C02F1/5245C02F2001/007C02F1/001C02F2103/38C02F2209/02C02F2209/08C02F2209/10C02F2301/08C02F1/004C02F1/76C02F2101/34C02F1/66C02F1/725C02F2103/10C02F2209/09C02F2303/02
Inventor 屈撑囤鱼涛李金灵杨博
Owner XI'AN PETROLEUM UNIVERSITY