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Composite material of silicon polymer and graphene oxide, high-strength impact-resistant epoxy resin material and preparation method thereof

A technology of composite materials and epoxy resin matrix, which is applied in the field of high-strength impact-resistant epoxy resin materials and its preparation, can solve the problems of high brittleness, high cross-linking density, and small molecular chain activity, so as to enhance toughness and improve The effect of tensile strength

Active Publication Date: 2021-08-20
JIAXING UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, after EP is cured, the crosslinking density is large, the dispersion is large, the molecular chain mobility is small, the material has low toughness, high brittleness, easy to crack, and poor impact resistance and peeling resistance, which limits its application range. The development of impact epoxy resin materials has important practical significance

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0024] The preparation method of the composite material of silicon polymer and graphene oxide comprises the following steps: reacting the silicon polymer and the graphene oxide dispersion liquid of tetrahydrofuran at a temperature of 60° C. for 5 hours to obtain the product. The mass ratio of graphene oxide in the graphene oxide dispersion liquid is 0.3:0.05, wherein the mass percentage of graphene oxide in the tetrahydrofuran graphene oxide dispersion liquid is 0.1%.

[0025] The diameter of graphene oxide in the graphene oxide dispersion in tetrahydrofuran is 100 nm.

[0026] The silicon polymer is prepared by the following method:

[0027] SiO was added to aqueous sodium hydroxide solution at room temperature 2 , then stirred and reacted for 3h, then added HCl, THF and NaCl to react for 30min, then stood still for 10min to obtain the upper layer organic solution, then dehydrated, suction filtered, and distilled to obtain the silicon polymer;

[0028] The concentration of ...

Embodiment 2

[0036] A method for preparing a composite material of a silicon polymer and graphene oxide, comprising the following steps: reacting a silicon polymer and a graphene oxide dispersion liquid of tetrahydrofuran at a temperature of 75°C for 4 hours, and the silicon polymer and tetrahydrofuran The mass ratio of graphene oxide in the graphene oxide dispersion liquid is 0.3:0.5, wherein the mass percentage of graphene oxide in the tetrahydrofuran graphene oxide dispersion liquid is 0.5%.

[0037] The diameter of graphene oxide in the graphene oxide dispersion in tetrahydrofuran was 5 μm.

[0038] The silicon polymer is prepared by the following method:

[0039] SiO was added to aqueous sodium hydroxide solution at room temperature 2 , then stirred and reacted for 4h, then added HCl, THF and NaCl to react for 30min, then stood still for more than 10min to obtain the upper layer organic solution, then dehydrated, suction filtered, and distilled to obtain the silicon polymer;

[0040...

Embodiment 3

[0049] A method for preparing a composite material of a silicon polymer and graphene oxide, comprising the following steps: reacting a silicon polymer and a graphene oxide dispersion liquid of tetrahydrofuran at a temperature of 70° C. for 4.5 hours, and the silicon polymer and tetrahydrofuran The mass ratio of graphene oxide in the graphene oxide dispersion liquid is 0.3:0.1, wherein the mass percentage of graphene oxide in the graphene oxide dispersion liquid in tetrahydrofuran is 0.2%.

[0050]The diameter of graphene oxide in the graphene oxide dispersion liquid in tetrahydrofuran was 1 μm.

[0051] The silicon polymer is prepared by the following method:

[0052] SiO was added to aqueous sodium hydroxide solution at room temperature 2 , then stirred and reacted for 3.5h, then added HCl, tetrahydrofuran and NaCl to react for 30min, then stood still for more than 10min to obtain the upper layer organic solution, then dehydrated, suction filtered, and distilled to obtain th...

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Abstract

The invention relates to a composite material of a silicon polymer and graphene oxide, a high-strength impact-resistant epoxy resin material and a preparation method thereof. The preparation method of the composite material of the silicon polymer and the graphene oxide comprises the steps of enabling the silicon polymer and a graphene oxide dispersion liquid of tetrahydrofuran to react for 4-5 h at the temperature of 60-75 DEG C, wherein the mass ratio of the silicon polymer to the graphene oxide in the graphene oxide dispersion liquid of the tetrahydrofuran is 0.3: (0.05-0.5), and the mass percentage content of graphene oxide in the graphene oxide dispersion liquid of tetrahydrofuran is 0.1%-0.5%. The invention prepares a composite material of a silicon polymer and graphene oxide. When the prepared composite material of the silicon polymer and the graphene oxide is applied to an epoxy resin material, the tensile strength of the epoxy resin can be improved, and the toughness of the epoxy resin can be enhanced.

Description

technical field [0001] The invention relates to a composite material of silicon polymer and graphene oxide, a high-strength impact-resistant epoxy resin material and a preparation method thereof. Background technique [0002] Epoxy resin (EP) refers to an organic polymer compound containing 2 or more epoxy groups in the molecule. Because of its high hardness, good flexibility, small curing shrinkage, strong adhesion and easy processing, It is widely used in the fields of automobile, construction, electronics, aerospace and thermosetting materials. However, after EP is cured, the crosslinking density is large, the dispersion is large, the molecular chain mobility is small, the material has low toughness, high brittleness, easy to crack, and poor impact resistance and peeling resistance, which limits its application range. The development of impact epoxy resin materials has important practical significance. [0003] The main methods to improve the toughness of epoxy resin ar...

Claims

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Application Information

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IPC IPC(8): C08K3/36C08K3/04C08L63/00
CPCC08K3/36C08K3/042C08K2201/005C08L63/00
Inventor 沈小军叶蓓党蕊琼施依呈张兰王永乐
Owner JIAXING UNIV