Adamantanecarboxylic acid benzyl amide derivative compound and skin whitening composition comprising same
A kind of adamantane carboxylic acid benzyl amide and skin whitening technology, which is applied in the preparation of carboxylic acid amide, the preparation of organic compounds, drug combination, etc., can solve the problems of insufficient whitening effect and limited use of stability problems, and solve the problem of fat The effect of excessive solubility increase
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[0064] The exemplary implementation example of this description is the preparation method of adamantane carboxylic acid benzyl amide derivative compound, as the preparation method of the adamantane carboxylic acid benzyl amide derivative compound, comprising: making adamantane-1-carboxylic acid and Steps in which the hydroxybenzylamine derivative reacts.
[0065] In an implementation example, the hydroxybenzylamine derivative can be selected from 2,4-dihydroxy-benzylbenzylamine, 3,4-dihydroxybenzylamine, 3,5-dihydroxybenzylamine, 2,5 - Any one of the group consisting of dihydroxybenzylamine, 4-hydroxybenzylamine, 3-hydroxybenzylamine and 2-hydroxybenzylamine.
[0066] Specifically, the adamantane-1-carboxylic acid can be dissolved in dichloromethane, and EDC (N-(3-dimethylaminopropyl)-N'ethylcarbodiimide hydrochloride ), in the presence of triethylamine, the hydroxybenzylamine derivative is reacted. In addition, after the reaction is finished, the compound represented by the...
Embodiment 1
[0093] [Example 1] Preparation of adamantane-1-carboxylic acid 2,4-dihydroxy-benzylamide
[0094]
[0095] The adamantane-1-carboxylic acid (1.8g) was dissolved in dichloromethane (50mL), and EDC (N-(3-dimethylaminopropyl)-N'ethyl carbon After diimine hydrochloride, 2.1 g), triethylamine (1.6 mL) and 2,4-dihydroxybenzylamine (1.4 g), it was stirred at normal temperature for 5 hours. After the reaction was completed, the reaction solution was washed with water and a saturated aqueous sodium chloride solution, and then the organic layer was dried with anhydrous magnesium sulfate. After the organic layer was concentrated under reduced pressure by filtration, it was separated by chromatography, whereby the chemical adamantane-1-carboxylic acid 2,4-dihydroxy-benzylamide (1.0 g) was harvested
[0096] 1 H NMR (300MHz, DMSO-d 6 )δ9.56(brs,1H),9.11(brs,1H),7.88(brs,1H),6.79(d,J=7.8Hz,1H),6.21(s,1H),6.15(d,J=7.8 Hz, 1H), 4.05(d, J=5.7Hz, 2H), 1.96~1.65(m, 15H).
Embodiment 2
[0097] [Example 2] Preparation of adamantane-1-carboxylic acid 3,4-dihydroxy-benzylamide
[0098]
[0099] Except having used 3,4-dihydroxybenzylamine instead of 2,4-dihydroxybenzylamine, the objective compound (1.6g) was harvested as a solid by substantially the same method as Example 1.
[0100] 1 H NMR (300MHz, DMSO-d 6 )δ8.71(brs,2H),7.77(brs,1H),6.63~6.59(m,2H),6.44(d,J=7.8Hz,1H),4.07(d,J=5.7Hz,2H), 1.96~1.65(m,15H).
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