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Hydrocracking catalyst

A hydrocracking and catalyst technology, applied in physical/chemical process catalysts, molecular sieve catalysts, inorganic chemistry, etc., can solve the problems of reduced active surface area and reduced unit cell size

Inactive Publication Date: 2006-01-04
SHELL INT RES MAATSCHAPPIJ BV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0006] In most of the dealumination treatments described in the literature, the treatment usually results in not only a reduction in the unit cell size but also a reduction in the active surface area

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0057] In the preparation of the catalyst according to the invention, after mixing the zeolite with the binder and, if present, the second cracking component, an aqueous acid solution can be added to the mixture after it has been milled, extruded and calcined in a conventional manner. Any suitable monobasic acid can be used as the acid solution, such as nitric acid and acetic acid. During extrusion, conventional extrusion aids can be used; commonly used extrusion aids include Superfloc available from Nalco.

[0058] Extrusion can be carried out using any conventional commercially available extruder. Specifically, a screw extruder can be used to force the mixture through holes in a die plate to produce a catalyst extrudate having a desired shape, such as a cylinder or a trilobal shape. The extruded die is then cut to the appropriate length. If desired, the catalyst extrudate may be dried, for example at a temperature of 100-300° C. for 30 minutes to 3 hours, prior to calcinat...

Embodiment 1

[0121] In these first tests, the activity of a number of comparative catalysts was evaluated against the catalysts of the invention. The results are given in Table 3.

[0122] Table 3 shows: when using the ultra-stable zeolite Y material with higher unit cell size (higher than 24.40 Å) to prepare hydrocracking catalyst, with the change of unit cell size, surface area, SAR and micropore volume, No increase in activity (expressed as T demand): For a net conversion of 65 wt%, comparative catalysts A and B exhibit more or less the same temperature demand (T demand).

[0123] Those skilled in the art will generally appreciate that below a certain unit cell size, further reductions in the unit cell size of the zeolite support (expressed as a decrease in aluminum content - also expressed as an increase in SAR) will result in a loss of activity , that is, a higher temperature is necessary to achieve the same conversion rate. This expectation is indeed confirmed by Comparative Cataly...

Embodiment 2

[0131] In this example, the catalysts of the present invention were evaluated for their hydrocracking selectivity to middle distillate hydrocarbons.

[0132] Middle distillates are here understood to be hydrocarbons in the kerosene plus diesel boiling range.

[0133] In order to get a true comparison of selectivities between catalysts, it is necessary to compare the selectivities under conditions of constant stability, ie at the same T requirement. Therefore, Table 4 compares the product selectivity of the comparison catalyst and the catalyst of the present invention on this basis. The selectivity of the following products is specifically recorded: C 1 -C 4 Hydrocarbon, C 5 -150°C (naphtha) hydrocarbons and 150°C-370°C hydrocarbons (kerosene and diesel).

[0134] It can be seen that the product selectivity is very similar.

[0135] Catalyst number

[0136] 1 Properties of zeolites

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PUM

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Abstract

Hydrocracking catalyst composition comprising an optional metal hydrogenation component supported on a carrier comprising a zeolite of the faujasite structure having a unit cell size in the range of from 24.10 to 24.40 Å, a bulk silica to alumina ratio (SAR) above about 12, and a surface area of at least about 850 m2 / g as measured by the BET method and ATSM D4365-95 with nitrogen adsorption at a p / po value of 0.03.

Description

technical field [0001] The present invention relates to catalyst compositions and their use in hydrocracking. Background technique [0002] In today's world, hydroconversion processes are important in providing the important base fuels needed for everyday life. Due to the increasing need to utilize heavy crude feedstocks, the refining industry has turned to the application of hydrocracking processes to provide the light base fuels demanded by modern society. Modern hydrocracking catalysts are generally based on zeolitic materials, although amorphous hydrocracking catalysts can be used. [0003] Faujasite materials are a major class of zeolitic materials proposed for hydrocracking applications. Early findings indicate that modification of the base material to reduce unit cell size as described in US-A-3,130,007 can improve selectivity to the desired middle distillate (or middle barrel) product. For this purpose, a combination of steam calcination and dealumination (usually...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J29/08B01J29/80B01J29/14C10G47/16B01J29/12B01J29/16B01J29/70B01J35/00C10G47/20
CPCB01J2229/42B01J2229/36B01J29/7007B01J35/002B01J2229/40Y10S423/21B01J29/084B01J2229/20C10G47/16B01J2229/22B01J29/166B01J2229/16B01J2229/37B01J29/146B01J29/80B01J29/126C10G47/20B01J29/14B01J35/30B01J35/77B01J35/70B01J2235/15B01J29/08
Inventor E·J·克雷格滕C·奥维汉德
Owner SHELL INT RES MAATSCHAPPIJ BV