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Preparation and use of polysilicate granular material

A granular material, polyaluminosilicate technology, applied in fibrous fillers, textiles and papermaking, inorganic pigment treatment, etc., to achieve the effect of improving physical stability, good physical stability, and avoiding gelation

Active Publication Date: 2012-02-15
NALCO CO
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Furthermore, when colloidal silica or other silicates are modified by incorporating aluminum into the silicate framework, known benefits such as increased acidity are obtained, but these materials have a strong tendency to form gels, which is unfavorable

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0045] In this particular example, aluminum doped silicic acid was prepared by adding 88.6 g of aluminum chlorohydrate to 1160 g of the 7% silicic acid sol prepared above.

[0046] 1000 ml of deionized water was added to the reaction flask and heated to 90°C. The aluminum-doped acid sol was fed via a peristaltic pump at a rate of 4.6 ml / min for two hours with pumping paused for 15 minutes. After 15 minutes, 50 mL of concentrated ammonium hydroxide was added to raise the pH of the reaction mixture to approximately pH9. The addition of the aluminum-doped silicic acid was continued until 130 g of the added aluminum-doped silicic acid were fed into the system. During this time, the pH was monitored periodically and an additional amount of 20% ammonium hydroxide was added to maintain the pH of the material above 9.5. The total addition time was approximately 3 hours.

[0047] After completion of the feed of aluminum-doped silicic acid, the reaction was heated at 90°C for an addi...

Embodiment 2

[0053] The experiment of Example 1 was repeated, wherein the polyaluminosilicate was prepared in a manner analogous to Example 1, but containing 34% by weight of Al, based on the silica present 2 o 3 , SiO 2 :Al 2 o 3 The molar ratio is 4.99.

[0054] In this embodiment, tests similar to Example 1 showed a surface area of ​​238 m 2 / g, the pore volume is 0.95cc / gm, and the pore diameter is 160 angstroms.

[0055] Comparative Example 3

[0056] The experiment of Example 1 was repeated to prepare an aluminum doped acid sol by adding 100.28 g of aluminum chlorohydrate to 1,286 g of a 4.9% acid sol prepared as previously described. A "mother liquor" was prepared by adding 750 ml of deionized water to the reaction flask and heating to 90°C. The aluminum doped acid sol was added via a peristaltic pump at a rate of 5.0 ml per minute until the full amount of acid sol was fed. No pH adjustment was made during the reaction in order to keep the conditions slightly acidic. The re...

Embodiment 4

[0060] Another experiment similar to Example 1 was performed, except Al 2 o 3 10% on the percentage of silicate present and SiO 2 :Al 2 o 3 The molar ratio is 16.97.

[0061] The resulting particulate material was measured to have 537.7M 2 / g surface area, 0.84cc / gm pore volume and 62.6 angstrom pore diameter.

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Abstract

A method for preparing a granular material, comprising the steps of: optionally adding a silicic acid solution optionally doped with aluminum to Preformed nanoparticle slurries. This method obtains a dispersion of polysilicate particles. The pH of the dispersion is then raised to greater than 7 to stabilize / strengthen the particles of the particle dispersion. Optionally, the particles can be dried and have increased porosity and surface area.

Description

technical field [0001] The present invention generally relates to methods of making particulate materials. More specifically, the present invention relates to methods of preparing particulate materials by mixing a solution of silicic acid with preformed nanoparticles to create polysilicate linkages in the dispersion. Background technique [0002] Microfine silica is used as a catalyst support, as a binder or as a catalyst itself, especially when "doped" with aluminum or another metal, as an ink-absorbing coating on paper etc., as an ink for wine or juice clarification Filter material used, etc. However, improvements can be obtained if the agglomerated silicate particles have a porosity greater than that obtained using standard colloidal silica. Furthermore, when colloidal silica or other silicates are modified by incorporating aluminum into the silicate framework, known benefits such as increased acidity are obtained, but these materials have a strong tendency to form gels...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C09C1/30C09C3/06D21H27/28
Inventor 弗朗索瓦·巴特洛布赖恩·T·霍兰德约翰·M·克拉尼斯基金·M·朗迈克尔·A·诺姆巴沙夏·维尔兹大卫·P·沃克曼
Owner NALCO CO