Process for producing rigid polyurethane slab foam, rigid polyurethane slab foam, and heat-insulating material for piping
A technology of rigid polyurethane and a manufacturing method, which is applied to the manufacture of rigid polyurethane sheet foam, rigid polyurethane sheet foam and thermal insulation materials for pipelines, can solve the problem of high thermal conductivity, no thermal insulation effect and thermal insulation effect, Can not meet the problems of flame retardancy and dimensional stability, and achieve the effect of low thermal conductivity, excellent dimensional stability, and excellent flame retardancy
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[0096] Examples of the present invention are described below, however, the present invention is not limited to these Examples. In addition, hereinafter, unless otherwise specified, "%" and "part" represent "mass%" and "mass part" respectively. In addition, modifiers used in the following preparation examples are the following compounds.
[0097] (1) Specific modifier (d1): polyester polyol (number of functional groups=2, hydroxyl value=270 mgKOH / g, number average molecular weight=416) obtained by reacting diethylene glycol and phthalic acid. (2) Specific modifying agent (d2): polyester polyol obtained by reacting diethylene glycol with phthalic acid and adipic acid (number of functional groups=2, hydroxyl value=230mgKOH / g, number average molecular weight=488 ). (3) Specific modifier (d3): polyester polyol (number of functional groups=2, hydroxyl value=255 mgKOH / g, number average molecular weight=440) obtained by reacting diethylene glycol and phthalic acid.
[0098] (4) Mod...
preparation example 1
[0100] According to the formula shown in the following table 1, in the reaction vessel that is provided with stirrer, thermometer, cooler and nitrogen inlet pipe, drop into the MDI (a1) of 32.4 parts (contain the dinuclear body of 4,4'-MDI more than 70%) ), heated to 60° C., then added 12.4 parts of specific modifier (d1), and stirred the system at 60° C. for about 2 hours, thereby modifying MDI. Next, 55.2 parts of polymerized MDI (a2) was added and mixed to the reaction product (modified MDI), thereby obtaining 100.0 parts of component [A] (hereinafter referred to as "Ingredient [A-1]").
[0101] The obtained component [A-1] was a transparent liquid without turbidity, and its viscosity (25° C.) was 1050 mPa·s. The ratio of the dinuclear body (unmodified MDI molecule) contained in this component [A-1] was 40%. In addition, the ratio of the dinuclear body in the total amount (87.6 parts) of the MDI (a1) subjected to the modification treatment and the polymerized MDI (a2) mix...
preparation example 2
[0103] According to the formula shown in the following table 1, the input amount of MDI (a1) is changed to 36.3 parts, and the addition amount of specific modifier (d1) is changed to 8.5 parts to modify MDI. In addition, In the same manner as in Preparation Example 1, 100.0 parts of component [A] (hereinafter referred to as "component [A-2]") containing a modified polyisocyanate having an NCO content of 27.5% was obtained.
[0104] The obtained component [A-2] was a transparent liquid without turbidity, and its viscosity (25° C.) was 284 mPa·s. The content ratio of the dinuclear body (unmodified MDI molecule) in this component [A-2] was 48%. In addition, the ratio of the dinuclear body in the total amount (91.5 parts) of the MDI (a1) subjected to the modification treatment and the polymerized MDI (a2) mixed after modification was 64%.
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