Oxetane-cyclic epoxy compound, method of preparing the same, and composite sheet and display substrate
A technology of oxetane and epoxy compounds, which is applied in the field of composite sheets and display substrates using the composite sheets, can solve the problems of poor solubility and wettability, unsuitable flexible substrates, increased viscosity, etc. Long and good bending, low thermal expansion coefficient, low viscosity effect
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preparation example 1
[0072] Preparation Example 1: Synthesis of Oxetane-Cyclic Epoxy Compound
[0073] NaH (6.4g) and 150ml of DMF were placed in a 500ml flask and stirred. After lowering the temperature with an ice bath, cyclohexenylmethanol (15 g) was slowly added to the above mixture and stirred at room temperature for 15 minutes. After lowering the temperature with an ice bath again, oxetane chloride (14.5 g) was slowly added to the above mixture over 10 minutes and stirred at room temperature for 2 hours. After the reaction, the H 2 O was slowly added to the product to remove the activity of the remaining sodium hydride, and then with ether / H 2 O treatment three times. MgSO 4 The organic layer was placed, then filtered and the solvent was removed using an evaporator to obtain a colorless liquid cyclohexenyl oxetane in 93% yield.
[0074] 1 H NMR (500MHz, CDCl 3 ): δ=1.25-1.30(m, 1H), 1.31(s, 3H), 1.71-1.83(m, 2H), 1.88-1.97(m, 1H), 2.04-2.14(m, 3H), 3.35(dd , 2H, 5Hz, 2Hz), 3.48(s, 2H...
Embodiment 1
[0078] Embodiment 1: prepare composite sheet
[0079]4.9 g of the oxetane-cyclic epoxy compound synthesized in Preparation Example 1, 5.1 g of bisphenol A diglycidyl ether and 0.2 g of triaryl hexafluorosulfonium antimonate were thoroughly mixed. 10 g of E-glass fiberglass (product name: 3313, Nittobo Co., Ltd.) was injected into the mixture, and then the article was placed between release-treated glass substrates, and UV irradiation was performed on both sides of the substrates for 2 minutes, thereby producing A transparent composite sheet with a binder content of 50 wt% (resin content: 50 wt%). figure 2 Its TMA map is shown.
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