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Preparation method of light-weight ammonium polyphosphate/silicon dioxide composite flame retardant

A technology of composite flame retardant and ammonium polyphosphate, which is applied in the field of preparation of lightweight ammonium polyphosphate/silica composite flame retardant, can solve problems such as high density, achieve improved hygroscopicity and dispersibility, and low density Effect

Inactive Publication Date: 2013-06-05
HENAN UNIVERSITY OF TECHNOLOGY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

These modified ammonium polyphosphates have excellent performance, but their density is relatively high, so they are not very suitable for foam plastics

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0015] Example 1. At room temperature, add type I ammonium polyphosphate into water and stir to dissolve, the weight / volume ratio of ammonium polyphosphate to water is 1:15, then add tetraethyl orthosilicate to the above solution under stirring, wherein Ammonium polyphosphate and SiO 2 The weight ratio of ammonium polyphosphate is 1:2, and then hydrochloric acid is added to control the pH value of the system at 5. After stirring for 4 hours, the silica sol mixed solution of ammonium polyphosphate is obtained. The obtained sol was spray-dried at a spray temperature of 140° C. and a detection temperature of 110° C. to obtain a white powder. The prepared white powder was dried at 80°C for 24 hours, and then vacuum-dried at 60°C for 8 hours to obtain a lightweight ammonium polyphosphate / silicon dioxide composite flame-retardant material with a hollow microsphere structure.

Embodiment 2

[0016] Example 2. At room temperature, add type I ammonium polyphosphate into water and stir to dissolve, the weight / volume ratio of ammonium polyphosphate to water is 1:20, then add methyl orthosilicate to the above solution under stirring, wherein Ammonium polyphosphate and SiO 2 The weight ratio of ammonium polyphosphate is 1:3, and then sulfuric acid is added to control the pH value of the system at 5. After stirring for 5 hours, the silica sol mixed solution of ammonium polyphosphate is obtained. The obtained sol was spray-dried at a spray temperature of 180° C. and a detection temperature of 120° C. to obtain a white powder. The prepared white powder was dried at 90°C for 12 hours, and then vacuum-dried at 70°C for 6 hours to obtain a lightweight ammonium polyphosphate / silicon dioxide composite flame-retardant material with a hollow microsphere structure.

Embodiment 3

[0017] Example 3. At room temperature, add type I ammonium polyphosphate into water and stir to dissolve, the weight / volume ratio of ammonium polyphosphate to water is 1:30, then add orthosilicate to the above solution under stirring, wherein Ammonium polyphosphate and SiO 2 The weight ratio of ammonium polyphosphate is 1:8, and then hydrochloric acid is added to control the pH value of the system at 4. After stirring for 4 hours, the silica sol mixed solution of ammonium polyphosphate is obtained. The obtained sol was spray-dried at a spray temperature of 160° C. and a detection temperature of 120° C. to obtain a white powder. The prepared white powder was dried at 80°C for 8 hours, and then vacuum-dried at 60°C for 6 hours to obtain a lightweight ammonium polyphosphate / silicon dioxide composite flame-retardant material with a hollow microsphere structure.

[0018] At room temperature, add type I ammonium polyphosphate into water and stir to dissolve. The weight / volume ratio...

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PUM

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Abstract

The invention relates to a preparation method of a light-weight ammonium polyphosphate / silicon dioxide composite flame retardant, which is characterized by comprising the following steps: dissolving I-type ammonium polyphosphate in water, adding silane, and adding acid to hydrolyze the silane to generate silica sol, thereby obtaining an ammonium polyphosphate / silica sol mixed solution; and carrying out spray drying on the sol, and drying the product to obtain the ammonium polyphosphate / silicon dioxide composite flame-retardant material. The composite flame retardant prepared by the method provided by the invention is in a hollow microsphere structure, and thus, has the advantages of low density and favorable dispersity; the ammonium polyphosphate is carried by the silicon dioxide to be dispersed in the hollow microsphere shell wall, and thus, the composite flame retardant has the advantages of favorable moisture resistance and low migration tendency; and the composite flame retardant has excellent synergic flame-retardant and smoke inhibition functions, and can be widely used for flame retarding of various materials, and especially various foam plastics.

Description

technical field [0001] The invention belongs to the field of inorganic material preparation, and in particular relates to a preparation method of a light ammonium polyphosphate / silicon dioxide composite flame retardant. Background technique [0002] The halogen-free intumescent flame retardant (IFR) based on ammonium polyphosphate has become a hot spot in the current flame retardant technology research due to its non-toxic, low smoke, and no droplet dripping characteristics. Ammonium polyphosphate plays the role of heat insulation and oxygen insulation by forming a dense carbon layer, so as to achieve the purpose of flame retardancy. However, due to the low molecular weight of conventional ammonium polyphosphate, it has disadvantages such as high hygroscopicity, thermal stability and poor compatibility with materials, which limit its application range. At present, the modification of ammonium polyphosphate mainly includes two methods: increasing the degree of polymerization...

Claims

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Application Information

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IPC IPC(8): C08K7/26C08K3/36C08K3/32
Inventor 苗蔚程文喜宋伟强付慧坛程巧换李金玲彭进
Owner HENAN UNIVERSITY OF TECHNOLOGY