Heavy distillate oil selective hydrogenation catalyst and application thereof
A heavy distillate oil, selective hydrogenation technology, applied in the direction of metal/metal oxide/metal hydroxide catalyst, physical/chemical process catalyst, heterogeneous catalyst chemical elements, etc., can solve the problem of poor selectivity, limited application and Development and other issues, to achieve the effect of good catalytic performance
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Embodiment 1
[0072] 1. Vector preparation
[0073] Take by weighing 2700 grams of pseudo-boehmite equivalent to 2000 grams of alumina, 2400 grams of alumina, and 300 grams of asparagus powder, mix, then add 400 grams of polyvinyl alcohol aqueous solution (mass concentration is 5%), and the mass concentration is 68 % of nitric acid 120 grams, 5000 milliliters of water, extruded, the wet bar was dried at 110 DEG C for 4 hours and then roasted at 750 DEG C for 4 hours to obtain a cylindrical carrier with a length of 4 mm and a diameter of 1.4 mm.
[0074] 2. Catalyst preparation
[0075] Mix 1 L of the above-mentioned carrier with 920 g of nickel nitrate-cerium nitrate mixed aqueous solution containing 140 g of nickel and 10.5 g of cerium, dry at 110°C for 8 hours, bake at 250°C for 2 hours, then raise the temperature to 450°C for 4 hours, reduce, and prepare Obtain Ni-based catalyst. The specific composition of the catalyst is shown in Table 2.
[0076] 3. Catalyst evaluation
[0077] Th...
Embodiment 2
[0085] 1. Vector preparation
[0086] Take by weighing 2700 grams of pseudo-boehmite equivalent to 2000 grams of alumina, 2400 grams of alumina, and 300 grams of asparagus powder, mix, then add 400 grams of polyvinyl alcohol aqueous solution (mass concentration is 5%), and the mass concentration is 68 % of nitric acid 120 grams, 5000 milliliters of water, extruded, the wet bar was dried at 110 DEG C for 4 hours and then roasted at 750 DEG C for 4 hours to obtain a cylindrical carrier with a length of 4 mm and a diameter of 1.4 mm.
[0087] 2. Catalyst preparation
[0088] Mix 1 L of the above-mentioned carrier with 920 grams of nickel nitrate-silver nitrate mixed aqueous solution containing 140 grams of nickel and 10.5 grams of silver, dry at 110°C for 8 hours, bake at 250°C for 2 hours, then heat up to 450°C for 4 hours, reduce, and prepare Obtain Ni-based catalyst. The specific composition of the catalyst is shown in Table 2.
[0089] 3. Catalyst evaluation
[0090] The ...
Embodiment 3
[0098] 1. Vector preparation
[0099] Take by weighing 2700 grams of pseudo-boehmite equivalent to 2000 grams of alumina, 2400 grams of alumina, and 300 grams of asparagus powder, mix, then add 400 grams of polyvinyl alcohol aqueous solution (mass concentration is 5%), and the mass concentration is 68 % of nitric acid 120 grams, 5000 milliliters of water, extruded, the wet bar was dried at 110 DEG C for 4 hours and then roasted at 750 DEG C for 4 hours to obtain a cylindrical carrier with a length of 4 mm and a diameter of 1.4 mm.
[0100] 2. Catalyst preparation
[0101] Mix 1 L of the above-mentioned carrier with 920 grams of nickel nitrate-copper nitrate mixed aqueous solution containing 140 grams of nickel and 10.5 grams of copper, dry at 110°C for 8 hours, bake at 250°C for 2 hours, then heat up to 450°C for 4 hours, reduce, and prepare Obtain Ni-based catalyst. The specific composition of the catalyst is shown in Table 2.
[0102] 3. Catalyst evaluation
[0103] The ...
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