Cured product, optical member, lens, compound and curable composition
A technology of cured products and compounds, which can be used in the fields of compounds and curable compositions, cured products, lenses, and optical components, and can solve problems such as chromatic aberration
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[0251] Hereinafter, an Example and a comparative example are given and the characteristics of this invention are demonstrated more concretely. Materials, usage amounts, ratios, processing contents, processing procedures, etc. shown in the following examples can be appropriately changed within a range not departing from the spirit of the present invention. Therefore, the scope of the present invention should not be limitedly interpreted by the specific examples shown below.
[0252] [chemical formula 23]
Synthetic example 1
[0254]
[0255]
[0256] Compound (I-1D) was synthesized by the method described in "Journal of Chemical Crystallography" (1997); 27(9); p.515-526.
[0257]
[0258] Compound (I-4A) was synthesized according to the synthesis method of compound (I-4A) described in JP-A-2016-081035.
[0259]
[0260] 15.5g (67.4mmol) of carboxylic acid compound (I-4A), 185mL of ethyl acetate, 46mL of N,N-dimethylacetamide and 60mg of 2,6-di-tert-butyl-4-methyl Phenol was mixed, and the internal temperature was cooled to 0°C. To the mixture was added dropwise 7.75 g (65.1 mmol) of thionyl chloride at an internal temperature of 0 to 5°C. After stirring at 5°C for 60 minutes, a solution of 6.85 g (27.6 mmol) of compound (I-1D) and 52 mL of THF (tetrahydrofuran) was added dropwise at an internal temperature of 0 to 8°C.
[0261] Thereafter, 16.8 g of N,N-diisopropylethylamine was added dropwise at an internal temperature of 0 to 10°C. After stirring for 1 hour at an internal temperature of...
Synthetic example 2
[0265]
[0266]
[0267] Compound (III-3Db) was synthesized by the method described in "Journal of Organic Chemistry" (2004); 69(6); p.2164-2177.
[0268]
[0269] 5.0 g (15.3 mmol) of compound (III-3Db), 1.66 g (16.80 mmol) of methyl cyanoacetate, and 25 mL of isopropanol were mixed, and stirred under reflux for 3 hours. After cooling to room temperature, 50 mL of water was added to the mixture, and the precipitated crystals were filtered. The obtained crystals were washed with a mixed solution of water-isopropanol (10:1) and a 0.5N hydrochloric acid solution, dissolved in N,N-dimethylacetamide, and filtered. Water was added to the obtained filtrate, and the precipitated crystals were filtered to obtain 2.2 g (7.82 mmol) of compound (III-3D) (yield 51%).
[0270]
[0271] Compound (I-1D) in the synthesis method of compound (I-4) described in Example 1 was changed to compound (III-3D), and the compound ( III-3) (yield 86%).
[0272] 1 H-NMR (400MHz, CDCl 3 ): δ (...
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