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Prepn of isobutene oxysulfide

A technology for sulfurizing isobutylene and oxidants, which is applied in the preparation of organic compounds, chemical instruments and methods, organic chemistry, etc., can solve the problems of strong corrosion, decreased solubility, and poor solubility of metals, and achieve reduced oxidation depth and good extreme pressure Anti-wear and low corrosion effects

Inactive Publication Date: 2003-08-20
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The problems of these patented technologies are as follows: (1) The solubility of the product in lubricating oil is poor, which may be due to the deepening of oxidation under acidic conditions, and the poor solubility of sulfones and olefins in the base oil in the product The increase of polymer content leads to a decrease in solubility; (2) the product is highly corrosive to metals, which may be due to the deepening of oxidation, and more sulfoxides and sulfones are generated in the product, and sulfoxides and sulfones are corrosive to metals higher than sulfide

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0014] This example is to use hydrogen peroxide as an oxidizing agent to prepare oxidatively sulfurized isobutylene in a neutral medium.

[0015] Dissolve 120 g of sulfurized isobutylene (commercial product) in 150 ml of toluene solution. The above solution was added into a 500ml three-neck flask, and stirred at a constant speed at room temperature. Then 100g concentration of 15% hydrogen peroxide solution was slowly added into the three-necked flask. The temperature was raised to 70°C and reacted for 2 hours. After the reaction, the reaction solution is cooled to room temperature, and the reaction solution will be divided into two incompatible phases: the upper layer is an organic phase containing the product, and the lower layer is an aqueous phase. Separate the aqueous phase with a separatory funnel and add 0.5 g of MnO to the remaining organic phase 2 To remove unreacted hydrogen peroxide. Then add 10ml concentration of 10% Na 2 CO 3 solution to remove traces of orga...

example 2

[0017] In this example, oxygen is used as an oxidizing agent, and in alkaline medium, Fe 2 o 3 As a catalyst for the preparation of oxidatively sulfurized isobutylene.

[0018] Dissolve 156 g of sulfurized isobutylene (industrial product) in 200 ml of toluene solution, add it into a 500 ml three-necked flask, and stir at a constant speed at room temperature. 5ml of 10% NaHCO 3 solution and 0.5 g powdered Fe 2 o 3 sequentially added to the above solution. Oxygen is introduced, and the flow rate of oxygen is 1.5L / min. The temperature was raised to 70°C and reacted for 2 hours. After the reaction, the reaction solution was cooled to room temperature, and Fe was filtered out. 2 o 3 , the reaction solution will be divided into two incompatible phases: the upper layer is the organic phase containing the product, and the lower layer is the aqueous phase. Then the remaining organic phase was washed with water until the reaction liquid was neutral. The product was treated wit...

example 3

[0023] This example is about the comparison of the extreme pressure properties of oxidatively sulfurized isobutylene.

[0024] 2g of sulfurized isobutylene and the samples obtained in examples and comparative examples were respectively dissolved in 100g of lubricating oil, and the extreme pressure performance of sulfurized isobutylene was evaluated by a four-ball machine test and a high-speed Timken abrasion tester. Evaluation items include (1) sintering load P D / Kg; (2) Load P when the wear spot diameter is 1mm D1 / Kg; (3) High-speed Timken OK value / N. The test results are shown in Table 1.

[0025] P D / Kg

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PUM

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Abstract

The present invention provides two kinds of preparation process of isobutene oxysulfide. Under neutral or alkali condition, isobutene sulfide and oxidant are mixed fully and reacted at 20-100 deg.c for 0.5-8 hr with the product being collected. These two kinds of preparation process can lower the oxidation depth effectively, and compared with available technology, the product has ever higher extreme pressure wear resistance, ever high oil-solubility and ever less corrosion.

Description

technical field [0001] The invention relates to a preparation method of an extreme-pressure anti-wear additive for lubricating oil, more specifically, a preparation method of oxidative sulfurized isobutylene. technical background [0002] Patents such as US 5062976, US 4904402, US 4822504 and EP 0312258 disclose the preparation methods of oxidative sulfurized isobutylene used as extreme pressure and antiwear agents for lubricating oils, and the common feature is that the oxidation reaction is carried out under acidic conditions. The problems of these patented technologies are as follows: (1) The solubility of the product in lubricating oil is poor, which may be due to the deepening of oxidation under acidic conditions, and the poor solubility of sulfones and olefins in the base oil in the product The increase of polymer content leads to a decrease in solubility; (2) the product is highly corrosive to metals, which may be due to the deepening of oxidation, and more sulfoxides...

Claims

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Application Information

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IPC IPC(8): C07C5/46C07C11/09C07C315/02C07C317/08C10M135/04
Inventor 李洪军仇延生
Owner CHINA PETROLEUM & CHEM CORP