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Method for treating surface of copper foil of affluxion body in lithium ion batteries

A lithium-ion battery and surface treatment technology, which is applied in the field of surface treatment technology and current collector copper foil, can solve the problems of easy detachment of electrode attachments, low copper foil roughness, and easy corrosion and discoloration of copper foil, so as to improve the synergy of corrosion inhibition effect, the effect of uniform roughening shape and good brightness

Inactive Publication Date: 2008-07-02
北京中科天华科技发展有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] Due to the smooth surface and low roughness of untreated copper foil, the electrode attachments are easy to fall off when making electrode pole pieces. At the same time, the copper foil is easy to corrode and discolor during transportation and use, so the surface treatment of copper foil is necessary.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] Put the 18μm thick copper foil in the roughened electrolyte at a temperature of 25°C and a current density of 0.4A / cm 2 Under the condition of cathodic electrolysis for 10s, take it out, and rinse it with deionized water for 1 to 5 times; 2 Under the condition of cathodic electrolysis for 120s, take it out, and rinse it with deionized water for 1 to 5 times; then put it into the antirust treatment solution, perform antirust treatment for 300s at a temperature of 50°C, take it out, and wash it with water 1 to 5 times, and after drying, a copper foil with a dendritic structure on the surface and a roughness of Ra=0.44 μm is obtained.

[0027] The roughened electrolyte is composed of copper ions Cu with a concentration of 10g / l 2+ , sulfuric acid H with a concentration of 140g / l 2 SO 4 , the stannous ion Sn of concentration 0.25g / l 2+ and tungsten ion W with a concentration of 0.03g / l 6+ composition;

[0028] The covering electrolyte is composed of copper ions Cu wit...

Embodiment 2

[0032] Put the 18μm thick copper foil in the roughened electrolyte at a temperature of 25°C and a current density of 0.4A / cm 2 Under the condition of cathodic electrolysis for 10s, take it out, and rinse it with deionized water for 1 to 5 times; then put it in the covering electrolyte, at a temperature of 25°C, and a current density of 0.1A / cm 2Under the condition of cathodic electrolysis for 120s, take it out, and rinse it with deionized water for 1 to 5 times; then put it into the antirust treatment solution, perform antirust treatment for 300s at a temperature of 50°C, take it out, and wash it with water 1 to 5 times, and after drying, a copper foil with a dendritic structure on the surface and a roughness of Ra=0.47 μm is obtained.

[0033] The roughened electrolyte is composed of copper ions Cu with a concentration of 10g / l 2+ , sulfuric acid H with a concentration of 140g / l 2 SO 4 , the concentration of 0.5g / l stannous ion Sn 2+ and tungsten ion W with a concentratio...

Embodiment 3

[0038] Put the 18μm thick copper foil in the roughened electrolyte at a temperature of 25°C and a current density of 0.4A / cm 2 Under the condition of cathodic electrolysis for 10s, take it out, and rinse it with deionized water for 1 to 5 times; then put it in the covering electrolyte, at a temperature of 25°C, and a current density of 0.1A / cm 2 Under the condition of cathodic electrolysis for 120s, take it out, and rinse it with deionized water for 1 to 5 times; then put it into the antirust treatment solution, perform antirust treatment for 300s at a temperature of 50°C, take it out, and wash it with water 1 to 5 times, and after drying, a copper foil with a dendritic structure on the surface and a roughness of Ra=0.42 μm is obtained.

[0039] The roughened electrolyte is made of copper ions Cu with a concentration of 15g / l 2+ , sulfuric acid H with a concentration of 140g / l 2 SO 4 , the concentration of 0.5g / l stannous ion Sn 2+ and tungsten ion W with a concentration o...

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Abstract

The method carries out coarsing, overlay and anticorrosive treatments for surface of copper foil with thickness less than or equal to 18 micro in order to raise cohesive force between copper foil and active materials. Coarsing treatment is that cathodal electrolysis is carried out for copper foil for 5-15s, in coarsing treating liquid composed of copper ion, vitriol, stannous ion and tungsten ion under conditioon of 15-40 deg.C, and certain current density; taking foil out, and using deionized water to wash the treated foil. Overlay treatment is that electrolysis is carried out for copper foil for 30-150s, in overlay treating liquid under condition of 15-40 deg.C, and certain current density. Anticorrosive treatment is carried out in BTA under 15-50 deg.C for 150-300s, and using deionized water to wash the treated foil. Then, drying the foil obtains dendritic structured copper foil in roughness larger than and equalto 0.25 micro, and less than and equal to 0.60 micro.

Description

technical field [0001] The invention relates to a surface treatment process for electrolytic copper foil, more particularly, a surface treatment method for a current collector copper foil with a thickness of ≤18 μm for a high-performance lithium battery. Background technique [0002] In recent years, with the miniaturization of electronic equipment such as mobile phones, cameras, and notebook computers, secondary batteries with high energy density are required. Lithium-ion secondary batteries have high energy density, good charge-discharge cycle performance, High discharge voltage platform, low self-discharge rate, no memory effect and other advantages, so it is widely used. [0003] The manufacturing process of the electrode sheet of the lithium-ion battery is as follows: a certain proportion of positive or negative active materials, conductive agents, binders and solvents are fully mixed to obtain electrode attachments for adhering to the positive or negative electrodes, a...

Claims

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Application Information

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IPC IPC(8): H01M4/04H01M4/64B23H3/00H01M10/40H01M10/0525
CPCY02E60/122Y02E60/10
Inventor 张世超
Owner 北京中科天华科技发展有限公司