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Method for producing cochleiform carbon fiber with catalyst

A helical carbon fiber and catalyst technology, which is applied in chemical instruments and methods, physical/chemical process catalysts, fiber chemical characteristics, etc., can solve problems such as high cost, difficulty in controlling metal particle dispersion and particle size, and save production costs , Overcome the difficulty of controlling the dispersion and particle size of metal particles, and improve the growth efficiency

Inactive Publication Date: 2010-06-23
BEIJING UNIV OF CHEM TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The present invention is to provide a method for preparing helical carbon fibers with a catalyst, which overcomes the disadvantages of high production cost of traditional carbon fibers and difficulty in controlling the dispersion and particle size of metal particles of traditional catalysts.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0018] With 80ml deionized water, 0.7755g Ni(NO 3 ) 2 ·6H 2 O, 0.5002g Al(NO 3 ) 3 ·7H 2 After O is formulated into a salt solution, 0.7928g of urea is added to make a mixed solution. Put it into the liner of the polytetrafluoroethylene resin of 100ml, seal in the autoclave. Put it into an oven at 120°C for crystallization for 15 hours, and finally take out the liner. After the reaction was completed, it was suction filtered, washed twice with deionized water, and dried at 70° C. for 15 hours.

[0019] Put 50 mg of the hydrotalcite prepared above into a porcelain boat and put it into a quartz tube, pass in nitrogen gas (60ml / min), raise the temperature to 700°C at a rate of 2°C / min, keep it warm for 20min, and then continue to pass in acetylene for 1h (The flow rates of acetylene and nitrogen are 6ml / min and 60ml / min respectively), and finally cooled to room temperature with the furnace to obtain chiral helical carbon fibers. The two helical carbon nanofibers grown sym...

Embodiment 2

[0021] With 80ml deionized water, 0.3785g NiSO 4 ·6H 2 O, 0.0372g Cu(NO 3 ) 2 ·3H 2 O, 0.6506gMgCl 2 ·6H 2 O and 0.3863g AlCl 3 ·6H 2 After O is formulated into a salt solution, 1.5375g of urea is added to make a mixed solution. Put it into the liner of the polytetrafluoroethylene resin of 100ml, put into the autoclave and seal. Put it in an oven at 150°C for 24 hours for crystallization, and finally take out the liner. After the reaction, filter with suction, wash twice with deionized water, and dry at 70° C. for 20 hours.

[0022]Put 40 mg of the hydrotalcite prepared above into a porcelain boat and put it into a quartz tube, pass in nitrogen gas (65ml / min), raise the temperature to 700°C at a rate of 5°C / min, keep it warm for 30min, and then continue to pass in acetylene for 1h30min (The flow rates of acetylene and nitrogen are 6ml / min and 65ml / min respectively), and finally cooled to room temperature with the furnace to obtain chiral helical carbon fiber and doub...

Embodiment 3

[0024] With 80ml deionized water, 1.2836g NiCl 2 ·6H 2 O, 0.1498g CuSO 4 ·5H 2 O, 0.7503gAl(NO 3 ) 3 ·7H 2 O prepared into a salt solution and then added 1.5856g of urea to make a mixed solution. Put it into the liner of the polytetrafluoroethylene resin of 100ml, put into the autoclave and seal. Put it into an oven at 150°C for 20 hours of crystallization, and finally take out the liner. After the reaction was completed, it was filtered with suction, washed twice with deionized water, and dried at 60° C. for 15 hours.

[0025] Put 45 mg of the hydrotalcite prepared above into a porcelain boat and put it into a quartz tube, pass in nitrogen gas (60ml / min), raise the temperature to 500°C at a rate of 10°C / min, keep it warm for 50min, and then continue to pass in acetylene for 1h30min (The flow rates of acetylene and nitrogen are 6ml / min and 60ml / min respectively), and finally cool down to room temperature with the furnace to finally obtain double-helix carbon fiber form...

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Abstract

The invention relates to a method which uses a catalyzer for preparing a twist carbon fiber and pertains to the field of carbon fiber preparation techniques. 30 to 50mg of hydrotalcite catalyzer is spread in a porcelain boat and then put into a horizontal quartz tube installed in a tube style heating furnace and nitrogen is pumped in the tube with the flow speed of 60-70ml / min; the temperature raises to 500-700 DEG C with the speed of 2-10 DEG C per minute and preserved for 20-60 minutes; then the acetylene is pumped in the catalyzer with the flow speed of 6-10ml / min at the temperature of 500-700 DEG C for the growth of carbon fiber and reaction for 1-2 hours, then cooled to chamber temperature along with the furnace, so as to obtain the twist carbon fiber; the twist carbon fiber comprises twist, chiral spiral and double helix carbon fibers. The method has the advantages that only acetylene is taken as a reducing gas and a carbon source for the growth of twist carbon fiber; the production cost is saved and the pollution to the environment is reduced substantially while the growth efficiency is enhanced. The twist, chiral spiral and double helix carbon fibers with even structure are finally obtained and the yield is higher, reaching 400-800 percent.

Description

technical field [0001] The invention belongs to the technical field of carbon fiber preparation, in particular to a method for preparing helical carbon fiber with a catalyst. Background technique [0002] The special structural characteristics of helical carbon fiber make it have good elasticity, strong mechanical properties and impact resistance, etc. It has a wide range of potential applications in hydrogen storage, adsorption, microwave absorption, electricity, etc. Inorganic functional materials. Among them, helical carbon fiber, chiral helical carbon fiber and double helical carbon fiber are typical helical carbon fibers, and they all have certain differences in size, morphology, structure, and performance. [0003] The most common preparation method for helical carbon fibers is catalytic chemical vapor deposition, or CCVD. The CCVD method has the advantages of simple equipment, low cost and easy control of the reaction process. The active components of catalysts use...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): D01F9/127B01J21/16
Inventor 李峰张璐项顼邹鲁
Owner BEIJING UNIV OF CHEM TECH