Solar battery sealing member and solar battery module
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[0249] Hereinafter, although this invention is demonstrated concretely based on an Example, this invention is not limited to these Examples.
[0250] (1) Measurement method
[0251] [Content ratio of ethylene unit, α-olefin, and vinyl acetate unit]
[0252] After filtering the solution obtained by heating and dissolving 0.35 g of the sample in 2.0 ml of hexachlorobutadiene with a glass filter (G2), 0.5 ml of deuterated benzene was added, and the solution was placed in an NMR tube with an inner diameter of 10 mm. Use the JNM GX-400 NMR measurement device manufactured by JEOL at 120°C 13 C-NMR determination. The cumulative number of times is more than 8000 times. according to income 13 The C-NMR spectrum quantifies the content ratio of ethylene units in the copolymer and the content ratios of α-olefin and vinyl acetate units.
[0253] [MFR]
[0254]The MFR of the ethylene-α-olefin copolymer and the ethylene-vinyl acetate copolymer was measured in accordance with ASTM D1238...
Synthetic example 1
[0297]A toluene solution of methylalumoxane as a cocatalyst was supplied at a ratio of 8.0 mmol / hr to one supply port of a continuous polymerizer with an internal volume of 50 L equipped with a stirring blade, and a toluene solution of methylaluminoxane as a main catalyst was supplied at a ratio of 0.025 mmol / hr. A hexane slurry of (1,3-dimethylcyclopentadienyl)zirconium dichloride was supplied to a hexane solution of triisobutylaluminum at a ratio of 0.5 mmol / hr to be used as a catalyst solution and a polymerization solvent The dehydrated and purified n-hexane was continuously supplied so that the total amount of the dehydrated and purified n-hexane became 20 L / hr. At the same time, ethylene is continuously supplied at a ratio of 3kg / hr, 1-butene is continuously supplied at a ratio of 15kg / hr, and hydrogen is continuously supplied at a ratio of 5NL / hr to other supply ports of the polymerizer. At a polymerization temperature of 90°C, a total pressure of 3MPaG , The continuous ...
Synthetic example 2
[0299] Supply the hexane solution of [dimethyl (tert-butylamide) (tetramethyl-η5-cyclopentadienyl) silane] titanium dichloride as procatalyst with the ratio of 0.012mmol / hr respectively, with 0.05mmol The ratio of / hr supplies triphenyl carbon as a cocatalyst The toluene solution of (tetrapentafluorophenyl) borate is supplied to the hexane solution of triisobutylaluminum at the ratio of 0.4mmol / hr, and the 1-butene is supplied at the ratio of 5kg / hr to 100NL / hr An ethylene-α-olefin copolymer was obtained in the same manner as in Synthesis Example 1 above except that hydrogen was supplied in proportion. The yield was 1.3 kg / hr. The physical properties are shown in Table 1.
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