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Method for recycling selenium from electrolytic manganese anolyte

A technology of anolyte and electrolytic manganese, applied in the direction of electrolysis process, electrolysis components, improvement of process efficiency, etc., can solve the problems of difficulty in using recycled selenium, unsuitable for selenium recycling, etc., achieve good economic and environmental benefits, and reduce consumption , the effect of simple operation

Active Publication Date: 2015-01-28
GUANGXI UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Due to the large amount of electrolytic manganese anolyte, it is also difficult to recover selenium by this process
[0010] In summary, the methods reported in the existing literature are generally only aimed at the removal of selenium in wastewater, and are not suitable for the recovery and utilization of selenium in electrolytic manganese anolyte.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] The electrolytic manganese anolyte (the composition is shown in Table 1) was filtered to separate the suspended matter, the filtrate and the manganese powder were uniformly mixed in the reactor at a liquid-solid ratio of 5L / g, and the reaction was carried out at 25°C for 120min, and the selenium in the anolyte was removed. The rate was 97.4%. After filtering, the filtrate is sent to a compound tank for leaching of manganese ore. The filter residue was heated and pretreated at 90°C for 30min, mixed with hydrogen peroxide at a liquid-solid ratio of 0.2L / Kg, and reacted at 45°C for 60min. The dissolution rate of selenium in the residue was 98%. After filtration, the filtrate is returned to the electrolytic manganese production as a selenium additive; the filter residue after separation of selenium is sent to the manganese ore leaching process for use.

[0022] Table 1 Analysis of main components of electrolytic manganese anolyte

[0023] Composition (g / L)

Embodiment 2

[0025] The electrolytic manganese anolyte (the composition is shown in Table 1) was filtered to separate the suspended matter, the filtrate and manganese powder were uniformly mixed in the reactor according to the liquid-solid ratio of 15L / g, and the reaction was carried out at 45°C for 90min, and the selenium in the anolyte was removed. The rate is 98.5%. After filtering, the filtrate is sent to a compound tank for leaching of manganese ore. The filter residue was heated and pretreated at 80°C for 60min, mixed with hydrogen peroxide at a liquid-solid ratio of 1.0L / Kg, and reacted at 35°C for 20min. The selenium dissolution rate in the residue was 99.6%. After filtration, the filtrate is returned to the electrolytic manganese production as a selenium additive; the filter residue after separation of selenium is sent to the manganese ore leaching process for use.

Embodiment 3

[0027] The electrolytic manganese anolyte (the composition is shown in Table 1) was filtered to separate the suspended matter, the filtrate and manganese powder were uniformly mixed in the reactor according to the liquid-solid ratio of 25L / g, and the reaction was carried out at 65°C for 60min, and the selenium in the anolyte was removed. The rate is 95.5%. After filtering, the filtrate is sent to a compound tank for leaching of manganese ore. The filter residue was heated and pretreated at 60°C for 90min, mixed with hydrogen peroxide at a liquid-solid ratio of 1.8L / Kg, and reacted at 50°C for 50min. The selenium dissolution rate in the residue was 97.4%. After filtration, the filtrate is returned to the electrolytic manganese production as a selenium additive; the filter residue after separation of selenium is sent to the manganese ore leaching process for use.

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Abstract

The invention provides a novel method for effectively recycling selenium from an electrolytic manganese anolyte. The method comprises the following basic steps: the filtered anolyte is uniformly mixed with manganese powders according to a liquid-solid ratio of 5 L / g to 40 L / g, the reaction is carried out for 10 to 120 minutes within a temperature range of 25 to 95 DEG C, and the selenium removal rate of the anolyte is above 90 percent; a filtrate obtained through filtering is sent to a compound bath for leaching of manganese ores, filter residues are preprocessed for 30 to 120 minutes within the temperature range of 40 to 90 DEG C and then uniformly mixed with hydrogen peroxide according to a liquid-solid ratio of 0.2 L / g to 2.6 L / g, the reaction is carried out for 20 to 60 minutes within the temperature range of 25 to 50 DEG C, and the selenium dissolution rate is above 95 percent; a filtrate obtained through secondary filtering is sent back to electrolytic manganese production and used as a selenium additive, and filter residues are sent to a manganese ore leaching procedure. The method provided by the invention has the advantages of large solution processing capacity, no loss of effective constituents, simplicity and high efficiency of the process, and no emissions of pollutants, and is particularly suitable for separating and recycling the selenium from the electrolytic manganese anolyte.

Description

Technical field: [0001] The invention relates to a method for recycling selenium in electrolytic manganese anolyte, which is particularly suitable for reducing selenium in electrolytic manganese anolyte by using manganese powder, so that selenium forms elemental selenium and is separated from the anolyte; then the elemental selenium is oxidized with hydrogen peroxide to generate Selenous acid and selenic acid are used back in the production of electrolytic manganese, so as to achieve the purpose of recycling selenium. Background technique: [0002] At present, domestic electrolytic manganese production enterprises generally use selenium dioxide (SeO 2 ) as an additive to improve the current efficiency of the electrolysis process, increase the corrosion resistance, and promote the crystal transformation of manganese. Every ton of electrolytic manganese product needs to consume 0.8-2.0Kg of SeO 2 . Generally, about 60% of the selenium enters the product, 23% enters the anod...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C25C1/10C25C7/06
CPCC25C1/10C25C7/06Y02P10/20
Inventor 王雨红粟海锋黎雪华蒋佳鸾农敬义蓝姿柳
Owner GUANGXI UNIV