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Method for preparing surface-functionalized porous carbon super capacitor electrode material

A surface functionalization and supercapacitor technology, which is applied in the manufacture of hybrid capacitor electrodes and hybrid/electric double layer capacitors, etc., can solve the problems of short cycle life, poor conductivity of conductive polymers and transition metal oxides, and limit wide application. To achieve the effect of increasing the specific capacitance value

Inactive Publication Date: 2016-03-02
CHINA UNIV OF PETROLEUM (EAST CHINA)
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Electrode materials are one of the key factors determining the performance of supercapacitors. Conductive polymers and transition metal oxides have disadvantages such as poor conductivity and short cycle life, which limit their wide application.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0018] The preparation method of the surface-functionalized porous carbon supercapacitor electrode material in this example is as follows: 0.6g macroporous carbon powder is mixed with 60mlH2O2, ultrasonicated for 30 minutes, then immersed for 1 hour, stirred at room temperature for 2 hours, and then deionized The product was washed with water until the pH value was neutral, and vacuum-dried at 80° C. for 12 hours to obtain a solid product after oxidation treatment. Put the oxidized solid product in a homogeneous reactor, mix it with hydroquinone at a mass ratio of 1:7, add 50ml of water, and place the reactor in a homogeneous reactor at 90°C After reacting for 10 hours, the product was washed twice with deionized water, and then vacuum-dried for 12 hours to obtain a surface-functionalized porous carbon material.

[0019] Nitrogen adsorption test shows that the surface functionalized porous carbon has a specific surface area of ​​222.4m2 / g, of which the mesopore specific surfac...

Embodiment 2

[0021] The preparation method of the surface-functionalized porous carbon supercapacitor electrode material in this example is as follows: 0.6g macroporous carbon powder is mixed with 60ml concentrated H2SO4, ultrasonicated for 30 minutes, then immersed for 1 hour, heated in a water bath at a constant temperature of 40°C, and stirred for 2 hours, and then wash the product with deionized water until the pH value is neutral, and dry it in vacuum at 80° C. for 12 hours to obtain a solid product after oxidation treatment. Put the oxidized solid product in a homogeneous reactor, mix it with naphthoquinone at a mass ratio of 1:7, add 50ml of water, and place the reactor in a homogeneous reactor at 90°C for 10 Hours, the product was washed twice with deionized water, and then vacuum-dried for 12 hours to obtain a surface-functionalized porous carbon material.

[0022] Nitrogen adsorption test shows that the surface functionalized porous carbon has a specific surface area of ​​198.6m2...

Embodiment 3

[0024] The preparation method of the surface-functionalized porous carbon supercapacitor electrode material in this example is as follows: 0.6g of mesoporous carbon powder is mixed with 60ml of concentrated HNO3, ultrasonicated for 30 minutes, then immersed for 1 hour, heated in a water bath at a constant temperature of 60°C, and stirred for 2 hours, and then wash the product with deionized water until the pH value is neutral, and dry it in vacuum at 80° C. for 12 hours to obtain a solid product after oxidation treatment. Put the oxidized solid product in a homogeneous reactor, mix it with hydroquinone at a mass ratio of 1:7, add 50ml of water, and place the reactor in a homogeneous reactor at 90°C After reacting for 10 hours, the product was washed with deionized water for 3 times, and then vacuum-dried for 12 hours to obtain a surface-functionalized porous carbon material.

[0025] Nitrogen adsorption test shows that the surface functionalized porous carbon has a specific su...

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Abstract

The invention relates to a method for preparing a surface-functionalized porous carbon super capacitor electrode material, comprising the following steps: (1) mixing porous carbon with excess oxidant, and heating and stirring the mixture to obtain a solid product after oxidation treatment; and (2) putting the product after oxidation treatment in a reaction kettle lined with polytetrafluoroethylene, and mixing the product with aqueous solution of a modifying agent to make the product and the aqueous solution react with each other to finally obtain a surface-functionalized porous carbon material. The surface-functionalized porous carbon prepared by the technology of the invention is not confined to double-electric-layer energy storage. Through surface modification treatment, active groups of the load on the surface of the carbon material can be oxidized or reduced to produce a Faraday pseudo-capacitor. As the surface-functionalized porous carbon can have two energy storage modes at the same time, the specific capacitance value is increased significantly compared with a carbon material of the same specific surface area, and the maximum specific capacitance value is up to 509F / g.

Description

technical field [0001] The invention relates to a method for preparing a surface-functionalized porous carbon supercapacitor electrode material, and belongs to the technical field of capacitor electrode material preparation. Background technique [0002] Supercapacitors, also known as electrochemical capacitors, have increasingly become a research hotspot in the field of new energy. Supercapacitor is a new type of energy storage element whose performance is between traditional capacitor and chemical power supply. Compared with traditional capacitors, it can provide higher specific energy, which can reach farad level or even thousand farad level, and the energy density that can be stored is more than 100 times that of electrostatic capacitance. Compared with chemical batteries, it has higher power density, which can reach 300W / kg-5000W / kg, equivalent to 5-10 times of batteries. In addition, supercapacitors also have the advantages of fast charge and discharge speed, long cy...

Claims

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Application Information

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IPC IPC(8): H01G11/34H01G11/86
CPCY02E60/13
Inventor 高秀丽
Owner CHINA UNIV OF PETROLEUM (EAST CHINA)