Coated Article Manufacturing Method, Coating And Laminate
A manufacturing method and article technology, applied in the direction of coating, metal material coating process, gaseous chemical plating, etc., can solve problems such as stripes or corrugated appearance, and achieve improved leveling ability, excellent adhesion, and excellent weather resistance and wear resistance effects
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[0123] Synthesis examples, examples and comparative examples of the present invention are given below by way of illustration and not by way of limitation.
Synthetic example 1
[0125] Synthesis of Silicone Acrylate (I)
[0126]In a 2-liter flask equipped with a stirrer, a condenser with a Dean-Stark trap, a dropping funnel and a thermometer, 235 g (0.5 mol) of Methyl Silicate 51 (Colcoat Co., Ltd.), 0.1 g of TBT700 (Nippon Soda Co., Ltd.) and 0.6 g of di-tert-butylhydroxytoluene, and heated to 85°C. To this, 551 g (5 mol) of hydroxyethyl acrylate was added and reacted. Care was taken to distill off methanol (80 g). The reaction mixture was treated under heating and reduced pressure (100° C., 5 mm Hg) for 2 hours to obtain 606 g (yield, 95%) of silicone acrylate (I) as a colorless liquid. The viscosity is 73 mPa·s, the specific gravity is 1.223, the refractive index is 1.4630, and the number of acrylic functional groups included by design per molecule is 10 equivalents.
Synthetic example 2
[0128] Synthesis of Acrylic Polymers
[0129] Synthetic acrylic polymer used as a coating ingredient (β). A 2 liter flask equipped with a stirrer, condenser, dropping funnel and thermometer was charged with 33.7 g of diacetone alcohol and heated to 80° C. under nitrogen flow. Into it were successively dripped portions of both:
[0130] (1) By adding 20 g of γ-methacryloxypropyltrimethoxysilane (available from Shin-Etsu Chemical Co., Ltd. as "KBM-503"; which corresponds to monomer unit D; monomer The ratio of unit D in the polymer is 20wt%), 2-[2'-hydroxyl-5'-(2-methacryloyloxyethyl) phenyl]-2H-benzotriazole (can be obtained from Otsuka Chemical Co., Ltd. obtained as "RUVA-93"; it corresponds to the monomer unit E; the proportion of the monomer unit E in the polymer is 15% by weight), 60 g of methyl methacrylate (MMA) and 5 g Glycidyl methacrylate (GMA) (these correspond to the monomer unit F; the proportion of the monomer unit F in the polymer is 65 wt%), and 140 g of diace...
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