Co hydrogenation reaction method to produce light olefins
A low-carbon olefin and reaction technology, which is applied in the reaction field of CO hydrogenation to produce low-carbon olefins, can solve the problem of low catalyst selectivity, avoid structural instability and deactivation, and improve the selectivity.
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Embodiment 1
[0065] Weigh equivalent to 50 g MoO 3 The ammonium paramolybdate was dissolved in water to obtain 100 grams of impregnating solution, which was mixed with 50 grams of alumina (20-60 mesh), steamed at 80°C under stirring until no visible liquid was found, dried at 120°C for 12 hours, and dried at 550°C. °C in an air atmosphere for 5 hours to obtain a catalyst.
[0066] The catalyst composition and evaluation results are shown in Table 1.
Embodiment 2
[0068] Weigh equivalent to 50 g MoO 3 and MnO 2 Ammonium paramolybdate and manganese nitrate (the atomic ratio of Mo to Mn is 100:70) were dissolved in water to obtain 100 grams of impregnation solution, which was mixed with 50 grams of alumina (20-60 mesh) and stirred for 80 °C until there is no visible liquid, dried at 120 °C for 12 hours, and calcined in an air atmosphere at 550 °C for 5 hours to obtain the catalyst.
[0069] The catalyst composition and evaluation results are shown in Table 1.
Embodiment 3
[0074] Weigh equivalent to 50 g MoO 3 Ammonium paramolybdate and CuO and copper nitrate hexahydrate (where the atomic ratio of Mo to Cu is 100:70) are dissolved in water to obtain 100 grams of impregnating solution, and the impregnating solution is mixed with 50 grams of alumina (20-60 mesh) , steamed at 80°C under stirring until no visible liquid was found, dried at 120°C for 12 hours, and calcined at 550°C for 5 hours in an air atmosphere to obtain a catalyst.
[0075] The catalyst composition and evaluation results are shown in Table 1.
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