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Deoxidation catalyst as well as preparation method and application thereof

A deoxidation catalyst and catalyst technology, applied in chemical instruments and methods, metal/metal oxide/metal hydroxide catalysts, physical/chemical process catalysts, etc., can solve problems such as high energy consumption

Active Publication Date: 2019-05-21
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, non-noble metals are limited by their activity and need to be reacted at a higher temperature, which consumes a lot of energy.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] Preparation of modified silicon oxide: use equal volume impregnation method on silicon oxide (commercially available commodity, properties are as follows: specific surface 335m 2 / g, pore volume is 0.86ml / g) impregnated with Nd nitrate and nickel nitrate aqueous solution, the molar concentration of Nd and nickel metal ions in the solution is 0.5mol / L, after impregnation, dry and roast, the drying time is 1h, dry The temperature is 100°C; the calcination time is 2h, and the temperature is 900°C;

[0022] Preparation of cobalt-loaded silicon oxide: impregnate cobalt nitrate solution on the modified silicon oxide by equal volume impregnation method, dry and roast after impregnation, the drying time is 2 hours, and the drying temperature is 130 ° C; the roasting time is 4 hours, the temperature is 400°C;

[0023] The zirconium sulfate and cobalt-loaded silica are kneaded and formed, and then dried and calcined to obtain a deoxidation catalyst. The drying time is 4 hours an...

Embodiment 2

[0026] Preparation of modified silicon oxide: use equal volume impregnation method on silicon oxide (commercially available commodity, properties are as follows: specific surface 335m 2 / g, pore volume is 0.86ml / g) impregnated with Nd nitrate and nickel nitrate aqueous solution, the molar concentration of Nd and nickel metal ions in the solution is 1.5mol / L, after impregnation, dry and roast, the drying time is 2h, dry The temperature is 100°C; the calcination time is 8h, and the temperature is 700°C;

[0027] Preparation of cobalt-loaded silica: impregnate cobalt sulfate solution on the modified silica by equal volume impregnation method, dry and roast after impregnation, the drying time is 3 hours, and the drying temperature is 120°C; the roasting time is 5 hours, the temperature is 450°C;

[0028] The zirconium sulfate and cobalt-loaded silica are kneaded and formed, and then dried and calcined to obtain a deoxidation catalyst. The drying time is 4 hours and the drying tem...

Embodiment 3

[0031] Preparation of modified silicon oxide: use equal volume impregnation method on silicon oxide (commercially available commodity, properties are as follows: specific surface 335m 2 / g, pore volume is 0.86ml / g) impregnated with Nd nitrate and nickel nitrate aqueous solution, the molar concentration of Nd and nickel metal ions in the solution is 1mol / L, after impregnation, dry and roast, the drying time is 0.5h, dry The temperature is 130°C; the calcination time is 5h, and the temperature is 800°C;

[0032] Prepare cobalt-loaded silica: impregnate cobalt bromide solution on the modified silica by equal-volume impregnation, dry and roast after impregnation, the drying time is 4 hours, and the drying temperature is 100°C; the roasting time is 4 hours, The temperature is 500°C;

[0033] Preparation of cobalt-loaded silica: impregnate cobalt sulfate solution on the modified silica by equal volume impregnation method, dry and roast after impregnation, the drying time is 3 hours...

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Abstract

The invention discloses a deoxidation catalyst and a preparation method thereof. The preparation method of the deoxidation catalyst comprises the following steps: step (1) co-impregnating silicon oxide with a mixed solution containing Nd and nickel, and then drying and roasting at high temperature to prepare modified silica; step (2) supporting cobalt on the modified silica prepared in the step (1), drying and calcining to obtain cobalt-supported silica; and step (3) mixing and kneading zirconium sulfate and the cobalt-supported silica prepared in the step (3) for molding, drying and roastingto obtain the deoxidation catalyst. The deoxidation catalyst is used for coalbed methane deoxidation and has the advantages of high activity, low reaction temperature, simple preparation method, low cost and the like.

Description

technical field [0001] The invention relates to a deoxidation catalyst and its preparation method and application, in particular to a coal gas bed deoxidation composite catalyst and its preparation method and application. Background technique [0002] my country is a big coal producing country, and a large amount of coalbed methane with different concentrations will be produced every year due to coal production. Developing effective coalbed methane utilization technology and reducing direct methane emissions are the key to building an energy-saving and environmentally friendly sustainable development model in my country and creating a low-carbon economy. an integral part of the system. Combining energy conservation and emission reduction and the improvement of environmental requirements, effectively and reasonably develop coalbed methane, a low-grade energy source, and convert it into usable resources, expand the scope and scale of coalbed methane use, and improve the utiliza...

Claims

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Application Information

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IPC IPC(8): B01J23/847C10L3/00C10L3/10
Inventor 李杰张信伟倪向前王海洋
Owner CHINA PETROLEUM & CHEM CORP