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Method for recycling waste selective catalytic reduction (SCR) catalyst

An SCR catalyst and resource utilization technology, applied in catalyst activation/preparation, chemical instruments and methods, physical/chemical process catalysts, etc., can solve the problems of high cost and long process flow, and achieve low production cost, short process flow, The effect of increasing economic value

Inactive Publication Date: 2019-06-11
WUHAN UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This method also has the disadvantages of long process flow and high cost.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0019] A method for resource utilization of spent SCR catalysts. 20-28wt% activated waste SCR catalyst, 25-30wt% clay, 33-40wt% fly ash and 6-10wt% expansion agent are used as catalyst raw materials, mixed and ground until the particle size is less than 0.05 mm, namely A catalyst mixture is obtained.

[0020] Put the catalyst mixture into a disc granulator, spray water while rotating the disc until the catalyst mixture forms spherical catalyst particles with a particle size of 3 to 5 mm; then place the spherical catalyst particles at 105 to 110 drying under the condition of ℃, and then roasting under the condition of 1050-1100 ℃ for 15-25 minutes to prepare the ozone catalyst.

[0021] The preparation method of the activated waste SCR catalyst is as follows: the waste SCR catalyst is cleaned, washed with water and air-dried, crushed, ground to a particle size of less than 0.15 mm, and then placed in a muffle furnace at a rate of 4-6 °C / min. Raise the temperature to 680-710°C...

Embodiment 2

[0024] A method for resource utilization of spent SCR catalysts. 28-36wt% activated waste SCR catalyst, 30-35wt% clay, 21-28wt% fly ash and 7-11wt% expansion agent are used as catalyst raw materials, mixed and ground until the particle size is less than 0.05 mm, namely A catalyst mixture is obtained.

[0025] Put the catalyst mixture into a disc granulator, spray water while rotating the disc until the catalyst mixture forms spherical catalyst particles with a particle size of 3 to 5 mm; then place the spherical catalyst particles at 105 to 110 drying at 1080-1120°C for 18-27 minutes to prepare an ozone catalyst.

[0026] The preparation method of the activated waste SCR catalyst is as follows: the waste SCR catalyst is cleaned, washed with water and air-dried, crushed, ground to a particle size of less than 0.15 mm, and then placed in a muffle furnace at a rate of 4-6 °C / min. Raise the temperature to 685-712°C at a rate of 20-30 minutes, then raise the temperature to 785-81...

Embodiment 3

[0029] A method for resource utilization of spent SCR catalysts. 36-44wt% activated waste SCR catalyst, 15-20wt% clay, 27-34wt% fly ash and 8-12wt% expansion agent are used as catalyst raw materials, mixed and ground until the particle size is less than 0.05 mm, namely A catalyst mixture is obtained.

[0030] Put the catalyst mixture into a disc granulator, spray water while rotating the disc until the catalyst mixture forms spherical catalyst particles with a particle size of 3 to 5 mm; then place the spherical catalyst particles at 105 to 110 drying under the condition of ℃, and then roasting under the condition of 1120-1150 ℃ for 20-28 minutes to prepare the ozone catalyst.

[0031] The preparation method of the activated waste SCR catalyst is as follows: the waste SCR catalyst is cleaned, washed with water and air-dried, crushed, ground to a particle size of less than 0.15 mm, and then placed in a muffle furnace at a rate of 4-6 °C / min. Raise the temperature to 690-715°C...

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Abstract

The invention relates to a method for recycling a waste selective catalytic reduction (SCR) catalyst. The method comprises the following steps: taking 20-50 wt% of an activated waste SCR catalyst, 15-35 wt% of clay, 15-40 wt% of coal ash and 5-12 wt% of an expanding agent as a catalyst raw material, and carrying out mixing and grinding to obtain a catalyst mixture; putting the catalyst mixture into a disc granulator, and spraying water while rotating a disc until spherical catalyst particles with a particle size of 3-5 mm are formed; and then drying the spherical catalyst particles, and carrying out roasting at a temperature of 1050-1200 DEG C for 15-30 minutes to prepare the ozone catalyst. The ozone catalyst is used for pretreatment of refractory industrial wastewater or is used for deeptreatment of biochemical tail water of refractory industrial wastewater, and the refractory industrial wastewater is one of coking wastewater, printing and dyeing wastewater, pharmaceutical wastewater and wastewater of chemical industrial parks. The method has the characteristics that the process flow is short, production cost is low, and waste is treated by waste; and a new path is opened up forrecycling the waste SCR catalyst.

Description

technical field [0001] The invention belongs to the technical field of waste SCR catalyst regeneration and utilization. In particular, it relates to a method for recycling waste SCR catalysts. Background technique [0002] Selective catalytic reduction (selective catalytic reduction, SCR) has been widely used in coal-fired power plants, coking and sintering plants, etc. because of its high denitrification efficiency and low operating costs, and has been considered as the preferred flue gas denitrification method so far. The SCR denitrification catalyst gradually becomes deactivated after a period of actual operation and must be replaced. The main causes of catalyst deactivation are chemical poisoning, thermal sintering, clogging / fouling, abrasion and so on. [0003] Chemical poisoning is the main reason for the deactivation of SCR catalysts in coal-fired power plants. It is mainly because certain components in the coal diffuse into the pores of SCR catalysts and combine wi...

Claims

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Application Information

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IPC IPC(8): B01J37/08B01J37/00C02F1/72C02F1/78
Inventor 颜家保刘旭东汪坤贾彪俞丹青吴玲张江雷杨郭芬胡杰
Owner WUHAN UNIV OF SCI & TECH