Quaternary efficient photocatalytic nano material with memory effect, preparation method thereof and air purifier
A nanomaterial, photocatalytic technology, applied in chemical instruments and methods, botanical equipment and methods, separation methods, etc., can solve the problem of photocatalysts losing catalytic activity and other problems, achieve excellent antibacterial properties, improve catalytic activity, and have a wide range of applications Effect
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[0047] The present invention further proposes a method for preparing a quaternary high-efficiency photocatalytic nanomaterial with a "memory" effect as described above, please refer to figure 1 , the preparation method of the quaternary high-efficiency photocatalytic nanomaterial with "memory" effect proposed by the present invention comprises the following steps:
[0048] S10, the Cu(NO 3 ) 2 ·3H 2 O is dissolved in a mixed solvent of glycerol, ethanol and water, and urea is added to react under closed heating conditions to obtain a mixed solution.
[0049] In this step, Cu-Cu is mainly prepared 2 O binary material, Cu-Cu 2 Cu and Cu in O binary materials 2 O is fused together to form a substance similar to an alloy. Under the condition of airtight heating, urea is used as a reducing agent to reduce divalent copper to monovalent copper and elemental copper. The reaction can be carried out in an autoclave, for example, will contain Cu(NO 3 ) 2 ·3H 2 A solution of O, g...
Embodiment 1
[0080] (1) 5mmol of Cu(NO 3 ) 2 ·3H 2 O was dissolved in 30mL of a mixed solvent of glycerol, ethanol and water (volume ratio of glycerol, ethanol and water, 7:7:10), and 9mmol urea was added to form a mixture containing Cu(NO 3 ) 2 ·3H 2 O, the solution of glycerol, ethanol, water, and urea were added in a stainless steel autoclave lined with polytetrafluoroethylene, and then the autoclave was placed in an oven at 180° C. for 10 h to obtain a mixed solution;
[0081] (2) Separating the mixed liquid from solid to liquid to obtain a solid, washing the solid, and vacuum drying at 65°C for 12 hours to obtain the first intermediate;
[0082] (3) The first intermediate is placed in an ethanol solution, ultrasonicated for 5 minutes to form a dispersion, and K is added to the dispersion. 2 SnO 3 ·3H 2 Aqueous solution of O (wherein K 2 SnO 3 ·3H 2 The amount of substance of O is 0.03mmol), and after stirring for 10min, a suspension is obtained;
[0083] (4) Add ethyl aceta...
Embodiment 2
[0088] (1) 5mmol of Cu(NO 3 ) 2 ·3H 2 O was dissolved in 30mL of a mixed solvent of glycerol, ethanol and water (volume ratio of glycerol, ethanol and water, 7:7:10), and 9mmol urea was added to form a mixture containing Cu(NO 3 ) 2 ·3H 2 O, the solution of glycerol, ethanol, water, and urea were added in a stainless steel autoclave lined with polytetrafluoroethylene, and then the autoclave was placed in an oven at 180° C. for 10 h to obtain a mixed solution;
[0089] (2) Separating the mixed liquid from solid to liquid to obtain a solid, washing the solid, and vacuum drying at 65°C for 12 hours to obtain the first intermediate;
[0090] (3) The first intermediate is placed in an ethanol solution, ultrasonicated for 5 minutes to form a dispersion, and K is added to the dispersion. 2 SnO 3 ·3H 2 Aqueous solution of O (wherein K 2 SnO 3 ·3H 2 The amount of substance of O is 0.06mmol), and after stirring for 10min, a suspension is obtained;
[0091] (4) Add ethyl aceta...
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