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Single crystalline phase catalyst

A technology of catalysts and orthorhombic crystal phases, applied in the direction of heterogeneous catalyst chemical elements, catalyst activation/preparation, physical/chemical process catalysts, etc., can solve problems such as loss

Inactive Publication Date: 2006-06-07
ROHM & HAAS CO
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Although this method can separate the orthorhombic phase, it is not ideal because about one-third of the original sample is lost in the extraction

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0123] Ammonium heptamolybdate tetrahydrate (17.03 g), ammonium metavanadate (3.35 g) and telluric acid (5.09 g) were dissolved in 284 g of water with heating. The resulting orange solution was cooled to 40 °C. Oxalic acid dihydrate (0.97 g) was dissolved in a solution of 6.5% w / w niobium oxalate in water (99.33 g). The resulting niobium-containing solution was added to the orange solution, and then 100 mg of the material prepared in Comparative Example 1 was added to the mixed solution. The mixture was dried on a rotary evaporator and then under vacuum (6 mbar) overnight. The resulting precursor was sieved to remove >50 mesh fines and then fired in a flowing atmosphere as follows: In an air atmosphere, the precursor was heated at 10°C / min from room temperature to 275°C and held at 275°C for 1 hour ; the atmosphere was changed to argon; in the argon atmosphere, the precursor was heated at 2°C / min from 275°C to 600°C, and then held at 600°C for 2 hours. The X-ray diffraction...

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PUM

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Abstract

Selective production of orthorhombic phase mixed metal oxides in quantitative yields.

Description

technical field [0001] The present invention relates to the catalyst that is used for oxidizing alkane or the mixture of alkane and alkene into its corresponding unsaturated carboxylic acid by gas-phase catalytic oxidation, more particularly relates to the preparation method of said catalyst and the catalyst prepared by the method of the present invention A method in which the catalyst catalyzes the gas phase oxidation of alkanes or a mixture of alkanes and alkenes to corresponding unsaturated carboxylic acids. The present invention also relates to a method for producing corresponding unsaturated nitriles through gas-phase catalytic oxidation of paraffin or a mixture of paraffin and alkene by using the catalyst prepared by the catalyst preparation method of the present invention in the presence of ammonia. Background technique [0002] Nitriles such as acrylonitrile and methacrylonitrile are produced industrially as important intermediates for the preparation of fibers, synt...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C07C253/24C07C51/16B01J27/057B01J23/00C01G39/00B01J23/20B01J23/28B01J23/887B01J37/02B01J37/04B01J37/08C07B61/00C07C51/215C07C57/05C07C253/26C07C255/08
CPCB01J23/002B01J23/20B01J23/28B01J27/0576B01J37/0236B01J37/08B01J2523/00C07C51/215C07C51/252C07C253/24C07C253/26Y02P20/52C07C57/04B01J2523/55B01J2523/56B01J2523/64B01J2523/68C07C255/08B01J27/057B01J23/887
Inventor L·E·小博根D·A·博斯F·A·P·卡瓦坎蒂M·B·小克拉克A·M·盖夫内S·汉
Owner ROHM & HAAS CO