Thermoelectric Element
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experiment 1
[0075] As starting materials, there were prepared Bi2Te3, Sb2Te3 and Bi2Se3 having an average particle diameter of 35 μm and a purity of not smaller than 99.99%.
[0076] To form an n-type thermoelectric element, the starting compounds were so weighed and mixed together as to form Bi2Te2.85Se0.15. Further, as a dopant, SbI3 was added in an amount of 0.09 parts by weight per 100 parts by weight of the sum of the starting compounds thereby to prepare a starting powder.
[0077] In order to form a p-type thermoelectric element, further, the starting compounds were so weighed and mixed together as to form Bi0.4Sb1.6Te3 to thereby prepare a starting powder.
[0078] The above starting powders were stirred in an isopropyl alcohol solvent by using a vibration mill for 5 to 72 hours, and the average particle diameter thereof was variously changed as shown in Table 1. The average particle diameter was found by measuring the particle size distribution after the treatment by using the vibration mill...
experiment 2
[0092] Various sintered bodies obtained in Experiment 1 were sliced into a predetermined thickness by using a wire saw to cut out wafers. A nickel electrode and a gold electrode were formed on the wafers by plating, and the wafers were cut into predetermined chips to obtain thermoelectric elements having electrodes.
[0093] The thermoelectric elements were arranged on an alumina ceramic insulating substrate (6 mm deep and 8.2 mm wide) having a copper electrode on the surface thereof, and were secured to the copper electrode via a solder layer in order to fabricate thermoelectric modules having shape factors L / S, element densities d and the shortest distances D among the elements as shown in Table 2.
[0094] While changing the current fed to the thermoelectric elements, the thermoelectric modules were measured for their maximum currents Imax with which the heat-generating member absorbs the heat in the greatest amount, and the maximum heat-absorbing amounts Qcmax. The results were as s...
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