Metallic compositions useful for brazing, and related processes and devices

Abstract

A braze alloy composition is disclosed, containing nickel, about 5% to about 40% of at least one refractory metal selected from niobium, tantalum, or molybdenum; about 2% to about 32% chromium; and about 0.5% to about 10% of at least one active metal element. An electrochemical cell that includes two components joined to each other by such a braze composition is also described. A method for joining components such as those within an electrochemical cell is also described. The method includes the step of introducing a braze alloy composition between a first component and a second component to be joined, to form a brazing structure. In many instances, one component is formed of a ceramic, while the other is formed of a metal or metal alloy.

Description

CROSS REFERENCE TO RELATED APPLICATIONS[0001]This application relates to, and claims priority from, the provisionally filed U.S. patent application Ser. No. 61 / 651,817, entitled “Compositions for Brazing, and Related Methods and Devices”, filed on May 25, 2012, which application is hereby incorporated by reference.TECHNICAL FIELD[0002]This invention generally relates to a braze composition. In some specific embodiments, the invention relates to a braze composition that provides corrosion-resistant sealing and other benefits to components used at high temperatures, e.g., thermal rechargeable batteries.BACKGROUND OF THE INVENTION[0003]A variety of electrochemical devices require processes and compositions for providing seals on or within the devices. The seals may be used to encapsulate the entire device, or they may separate various chambers within the device. As an example, many types of seal materials have been considered for use in high-temperature rechargeable batteries / cells for...

AI Technical Summary

Benefits of technology

[0008]In view of some of these concerns and challenges, it may be desirable to develop new braze alloy compositions that have properties and characteristics that meet performance requirements for high temperature rechargeable batteries, and are less complicated and less expensive to process, as compared to the existing sealing methods.

Problems solved by technology

While mechanisms for sealing these components are currently available, their use can sometimes present some difficulty.

For example, metal-to-ceramic bonding can be challenging, due to thermal stress caused by a mismatch in the coefficient of thermal expansion for the ceramic and metal components.

However, most of the seals may not be able to withstand high temperatures and corrosive environments.

In short, the method is relatively expensive, and complicated, in view of the multiple processing steps, and the difficulty in controlling the processing steps.

However, most of the brazing materials (or braze materials) have limitations that prevent them from fulfilling all of the necessary requirements of high temperature batteries.

Moreover, some of the commercial braze materials can be quite expensive themselves; and using them efficiently in various processes can also be costly.

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