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Method for preparing boron carbide composite material

A composite material and boron carbide technology, which is applied in the field of composite material preparation, can solve the problems of low density and high brittleness of boron carbide materials, and achieve the effects of low preparation environment and equipment requirements, increasing density and reducing production costs.

Inactive Publication Date: 2010-07-28
NORTHEASTERN UNIV LIAONING
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] The purpose of the present invention is to provide a method for preparing boron carbide composite materials for the problems of low density and high brittleness of pressureless sintered boron carbide materials

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0015] Example 1: Forming ingredients, adding TiO at a mass fraction of 30% 2 , its purity is 99wt%, the balance is B 4 C, the purity is 98wt%, of which A powder d 50 =1μm, B powder d 50 = 20 μm, A and B are added at a mass ratio of 0.25, mixed by ball milling, the medium is absolute ethanol, and the grinding balls are corundum balls. After the material is ball milled for 24 hours, it is dried at 60°C for 18 hours, and a phenolic resin-acetone solution binder is added according to 15% of the total mass fraction of the material. The content of phenolic resin in the binder is 50wt%, and then granulated with a 60-mesh sieve, and Molded at 150MPa, the formed sample was dried at 100°C for 12h.

[0016] Pressureless pre-firing, place the preform in a vacuum sintering furnace, evacuate to 100Pa, then raise the temperature to 2050 °C at a rate of 5 °C / min, and keep it for 30 min to obtain a boron carbide-based porous pre-sintered body.

[0017] Vacuum infiltration, the porous calc...

example 2

[0018] Example 2: Forming ingredients, adding TiO at a mass fraction of 50% 2 , its purity is 99wt%, the balance is B 4 C, the purity is 98wt%, of which A powder d 50 =1μm, B powder is d 50 = 20 μm, A and B are added at a mass ratio of 0.3, mixed by ball milling, the medium is absolute ethanol, and the grinding balls are corundum balls. After the material was ball milled for 24 hours, it was dried at 60°C for 18 hours, and a phenolic resin-acetone solution binder was added according to 15% of the mass fraction of the material. The content of phenolic resin in the binder was 50wt%, and then granulated with a 60-mesh sieve. Compression molding was performed under 150MPa, and the formed samples were dried at 100°C for 12 hours.

[0019] Pressureless pre-firing, place the preform in a vacuum sintering furnace, evacuate to 100Pa, then raise the temperature to 2050 °C at a rate of 5 °C / min, and keep it for 30 min to obtain a boron carbide-based porous pre-sintered body.

[0020]...

example 3

[0021] Example 3: Forming ingredients, adding ZrO at 5% mass fraction 2 , its purity is 99.5wt%, the balance is B 4 C, the purity is 99wt%, of which A powder d 50 =0.5μm, B powder d 50 =10 μm, A and B are added at a mass ratio of 0.1, mixed by ball milling, the medium is absolute ethanol, and the grinding balls are corundum balls. After the material was ball milled for 24 hours, it was dried at 60°C for 18 hours, and a phenolic resin-acetone solution binder was added according to 10% of the mass fraction of the material. The content of phenolic resin in the binder was 50wt%, and then granulated with a 24-mesh sieve. Compression molding was performed under 100MPa, and the formed samples were dried at 100°C for 12 hours.

[0022] Pressureless pre-firing, the preform is placed in a vacuum sintering furnace, vacuumed to 50Pa, then heated to 2060 °C at a rate of 8 °C / min, and kept for 60 min to obtain a boron carbide-based porous pre-sintered body.

[0023] Vacuum infiltration,...

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PUM

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Abstract

The invention relates to a process for preparing boron carbide composite material, which is characterized in that the steps comprise that metal oxide powder is taken 5%-50% by mass percentage and the left is boron carbide powder, blending and die-pressing the mixture into performs at 100-150MPa, then, laying the performs in the vacuum sintering furnace, vacuumizing to 20-100Pa, heating up to 1850-2060DEG C by the speed of 5-8DEG C / min and insulating 10-60 minutes, porous boron carbide preburning body is obtained, at last, infiltrating aluminum under vacuum, infiltration technique is 900-1100DEG C, thermal insulation time is 0.5-2h, and evacuation is 5-100Pa. The invention improves fracture toughness property by 1.78-2.75 times on the basis of single boron carbide materials. Further, the invention has the advantages that the manufacturing cost is low and the process for preparation is simple, which is in favor of being processed into variety of complicated products and is easy to be popularized and applied in the production field of boron carbide ceramics materials.

Description

technical field [0001] The invention relates to a preparation method of a composite material, in particular to a preparation method of a boron carbide composite material. Background technique [0002] Boron carbide has the characteristics of low density, good acid and alkali corrosion resistance, strong neutron absorption capacity, and also has super high hardness, especially its constant high temperature hardness is unmatched by other materials. It is the content of key development in the fields of friction products, nuclear industry neutron protection materials, bulletproof materials and other fields. [0003] At present, there are two methods for manufacturing boron carbide ceramic materials: pressureless sintering and hot pressing sintering. The density of boron carbide products manufactured by pressureless sintering is low, so that its technical performance indicators cannot meet the requirements of various products. Adding second-phase particles in boron carbide can ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C04B35/563C04B35/622C04B41/88
Inventor 茹红强吕鹏喻亮左良孙旭东
Owner NORTHEASTERN UNIV LIAONING