Fire resistant water resistant polyurethane composition for fluid sealant and manufacture method thereof
A technology of high temperature resistance and polyurethane, applied in the field of polyurethane composition for sealant and its preparation
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Embodiment 1
[0032] The raw materials and their consumption are:
[0033] 90 parts by mass of polyisocyanate prepolymer (1,4-cyclohexane diisocyanate (CHDI) / polyoxypropylene glycol (molecular weight 6000) / dioctyl phthalate (DOP) / stannous octoate),
[0034] 1 mass part multifunctional grafting monomer (A is amino, B is epoxy, OR' is methoxyl group),
[0035] 10 parts by mass of high temperature resistant compound (epoxy resin E-51).
[0036] The preparation method is as follows:
[0037] (a) Preparation of polyisocyanate prepolymer
[0038] Add 272g of DOP and 1000g of polyoxypropylene diol into the reaction kettle, and dehydrate under vacuum at 110°C-120°C for 1 hour. The temperature was lowered to 50°C, 105g of CHDI and 0.01g of stannous octoate were added, and the temperature was raised to 70°C to react for 1 hour. The measured NCO% was 3.0%, and the viscosity was 6050 mPa·s.
[0039] (b) Reaction of polyisocyanate prepolymer with multifunctional graft monomer
[0040] Mix the poly...
Embodiment 2
[0049] The raw materials and their consumption are:
[0050] 80 parts by mass of polyisocyanate prepolymer (diphenylmethane-4,4'-diisocyanate (MDI) / polycarbonate diol (molecular weight 2000) / diisononyl phthalate (DINP) / dilauric acid Di-n-butyltin),
[0051] 5 parts by mass of multifunctional grafting monomer (A is amino, B is vinyl, OR' is methoxyl group),
[0052] 5 parts by mass of high temperature resistant compound (bismaleimide).
[0053] The preparation method is as follows:
[0054] (a) Preparation of polyisocyanate prepolymer
[0055] Add 52g of diisononyl phthalate (DINP) and 2000g of polycarbonate diol into the reaction kettle, and vacuum dehydrate at 110°C to 120°C for 1 hour. Cool down to 50°C, add 400g of MDI and 0.02g of di-n-butyltin dilaurate, and raise the temperature to 70°C for 1 hour. The measured NCO% is 2.02%, and the viscosity is 9500mPa·s.
[0056] (b) Reaction of polyisocyanate prepolymer with multifunctional graft monomer
[0057] Mix according...
Embodiment 3
[0066] The raw materials and their consumption are:
[0067] Polyisocyanate prepolymer (isophorone diisocyanate (IPDI) / polycaprolactone diol (molecular weight 3000) / didecyl phthalate (DIDP) / di-n-butyltin dilaurate) 60 parts by mass, more 5 parts by mass of functional grafting monomer (A is amino group, B is vinyl group, OR' is ethoxy group), and 20 parts by mass of high temperature resistant compound (nano-silica hybrid acrylic resin).
[0068] The preparation method is as follows:
[0069] Preparation of polyisocyanate prepolymer
[0070] Add 1159g didecyl phthalate (DIDP) and 1500g polycaprolactone diol into the reaction kettle, and vacuum dehydrate at 110°C-120°C for 1 hour. Cool down to 50°C, add 334g IPDI and 0.015g di-n-butyltin dilaurate, and raise the temperature to 80°C for 1 hour. The measured NCO% is 2.76%, and the viscosity is 7000mPa·s.
[0071] (b) Reaction of polyisocyanate prepolymer with multifunctional graft monomer
[0072] Mix according to the ratio, r...
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